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Solid-state solar modules based on mesoscopic organometal halide perovskite: a route towards the up-scaling process
Abstract
We fabricated the first solid state modules based on organometal halide perovskite CH3NH3PbI3-xClx using Spiro-OMeTAD and poly(3-hexylthiophene) as hole transport materials. Device up-scaling was performed using innovative procedures to realize large-area cells and the integrated series-interconnections. The perovskite-based modules show a maximum conversion efficiency of 5.1% using both poly(3-hexylthiophene) and Spiro-OMeTAD. A long-term stability test was performed (in air, under AM1.5G, 1 Sun illumination conditions) using both materials showing different behaviour under continuous light stress. Whilst the poly(3-hexylthiophene)-based module efficiency drops by about 80% with respect to the initial value after 170 hours, the Spiro-based module shows a promising long-term stability maintaining more than 60% of its initial efficiency after 335 hours.
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Cited by
Stability of Metal Halide Perovskite Solar Cells
Leijtens, T., Eperon, G. E., Noel, N. K., Habisreutinger, S. N., Petrozza, A., & Snaith, H. J. (2015) · Advanced Energy Materials · doi:10.1002/aenm.201500963 · Cited by 1,308
Benefits of very thin PCBM and LiF layers for solution-processed p–i–n perovskite solar cells
Seo, J., Park, S., Chan Kim, Y., Jeon, N. J., Noh, J. H., Yoon, S. C., & Seok, S. I. (2014) · Energy Environ. Sci. · doi:10.1039/c4ee01216j · Cited by 677
Device stability of perovskite solar cells – A review
Asghar, M. I., Zhang, J., Wang, H., & Lund, P. D. (2017) · Renewable and Sustainable Energy Reviews · doi:10.1016/j.rser.2017.04.003 · Cited by 423
Razza, S., Di Giacomo, F., Matteocci, F., Cinà, L., Palma, A. L., Casaluci, S., Cameron, P., D'Epifanio, A., Licoccia, S., Reale, A., et al. (2015) · Journal of Power Sources · doi:10.1016/j.jpowsour.2014.12.008 · Cited by 384
Self-citationOrganic–inorganic halide perovskite/crystalline silicon four-terminal tandem solar cells
Löper, P., Moon, S.-J., Martín de Nicolas, S., Niesen, B., Ledinsky, M., Nicolay, S., Bailat, J., Yum, J.-H., De Wolf, S., & Ballif, C. (2015) · Physical Chemistry Chemical Physics · doi:10.1039/c4cp03788j · Cited by 367
Metadata
- Authors
- Matteocci, F., Razza, S., Di Giacomo, F., Casaluci, S., Mincuzzi, G., Brown, T. M., D'Epifanio, A., Licoccia, S., & Di Carlo, A.
- Venue
- Physical Chemistry Chemical Physics
- Publisher
- Royal Society of Chemistry (RSC)
- Published
- 2014
- Volume
- 16
- Issue
- 9
- Pages
- 3918
- ISSN
- 1463-9076 (ISSN-L)
- 1463-9084
- OpenAlex
- W2009244270
- Cited by
- 182
- References
- 0
- FWCI
- 15.74
- Type
- journal article
- Language
- en
- Open access
- closed
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- The paper
- Matteocci, F., Razza, S., Di Giacomo, F., Casaluci, S., Mincuzzi, G., Brown, T. M., D'Epifanio, A., Licoccia, S., & Di Carlo, A. (2014). Solid-state solar modules based on mesoscopic organometal halide perovskite: a route towards the up-scaling process. Physical Chemistry Chemical Physics. https://doi.org/10.1039/c3cp55313b
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