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High and anisotropic carrier mobility in experimentally possible Ti2CO2(MXene) monolayers and nanoribbons
Abstract
MXene, a new kind of two-dimensional (2D) material, has a unique combination of excellent physical and chemical properties. Via computations on density functional theory and deformation potential theory, we investigated the electronic structure and predicted the carrier mobility of Ti2CO2 (a typical MXene) monolayers and nanoribbons. The Ti2CO2 monolayer is a semiconductor with a band gap of 0.91 eV, and the hole mobility in the monolayer reaches 10(4) orders of magnitude along both x and y directions, which is much higher than that of MoS2, while the electron mobility is about two orders of magnitude lower. The dramatic difference between the hole and electron mobilities also exists in nanoribbons. Moreover, our results suggest that width controlling and edge engineering would be effective in adjusting the carrier mobility of Ti2CO2 nanoribbons, and endow experimentally available Ti2CO2 with wide applications to field-effect transistors and photocatalysts.
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Cites
Electronics and optoelectronics of two-dimensional transition metal dichalcogenides
Wang, Q. H., Kalantar-Zadeh, K., Kis, A., Coleman, J. N., & Strano, M. S. (2012) · Nature Nanotechnology · doi:10.1038/nnano.2012.193 · Cited by 16,374
Cited by
2D MXenes: A New Family of Promising Catalysts for the Hydrogen Evolution Reaction
Gao, G., O’Mullane, A. P., & Du, A. (2017) · ACS Catalysis · doi:10.1021/acscatal.6b02754 · Cited by 1,153
A Review on MXene Synthesis, Stability, and Photocatalytic Applications
Murali, G., Reddy Modigunta, J. K., Park, Y. H., Lee, J.-H., Rawal, J., Lee, S.-Y., In, I., & Park, S.-J. (2022) · ACS Nano · doi:10.1021/acsnano.2c04750 · Cited by 668
Recent advance in MXenes: A promising 2D material for catalysis, sensor and chemical adsorption
Zhu, J., Ha, E., Zhao, G., Zhou, Y., Huang, D., Yue, G., Hu, L., Sun, N., Wang, Y., Lee, L. Y. S., et al. (2017) · Coordination Chemistry Reviews · doi:10.1016/j.ccr.2017.09.012 · Cited by 659
Oxygen‐Functionalized Ultrathin Ti 3 C 2 T x MXene for Enhanced Electrocatalytic Hydrogen Evolution
Jiang, Y., Sun, T., Xie, X., Jiang, W., Li, J., Tian, B., & Su, C. (2019) · ChemSusChem · doi:10.1002/cssc.201803032 · Cited by 367
Chandrasekaran, A., Mishra, A., & Singh, A. K. (2017) · Nano Letters · doi:10.1021/acs.nanolett.7b01035 · Cited by 292
Metadata
- Authors
- Zhang, X., Zhao, X., Wu, D., Jing, Y., & Zhou, Z.
- Venue
- Nanoscale
- Publisher
- Royal Society of Chemistry (RSC)
- Published
- 2015
- Volume
- 7
- Issue
- 38
- Pages
- 16020-16025
- ISSN
- 2040-3364 (ISSN-L)
- 2040-3372
- OpenAlex
- W1950367212
- Cited by
- 290
- References
- 1
- FWCI
- 10.53
- Type
- journal article
- Language
- en
- Open access
- closed
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- Zhang, X., Zhao, X., Wu, D., Jing, Y., & Zhou, Z. (2015). High and anisotropic carrier mobility in experimentally possible Ti2CO2(MXene) monolayers and nanoribbons. Nanoscale. https://doi.org/10.1039/c5nr04717j
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