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Efficient vacuum deposited p-i-n and n-i-p perovskite solar cells employing doped charge transport layers
Open accessAbstract
Methylammonium lead halide perovskites have emerged as high performance photovoltaic materials. Most of these solar cells are prepared via solution-processing and record efficiencies (>20%) have been obtained employing perovskites with mixed halides and organic cations on (mesoscopic) metal oxides. Here, we demonstrate fully vacuum deposited planar perovskite solar cells by depositing methylammonium lead iodide in between intrinsic and doped organic charge transport molecules. Two configurations, one inverted with respect to the other, p-i-n and n-i-p, are prepared and optimized leading to planar solar cells without hysteresis and very high efficiencies, 16.5% and 20%, respectively. It is the first time that a direct comparison between these two opposite device configurations has been reported. These fully vacuum deposited solar cells, employing doped organic charge transport layers, validate for the first time vacuum based processing as a real alternative for perovskite solar cell preparation.
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Stranks, S. D., Eperon, G. E., Grancini, G., Menelaou, C., Alcocer, M. J. P., Leijtens, T., Herz, L. M., Petrozza, A., & Snaith, H. J. (2013) · Science · doi:10.1126/science.1243982 · Cited by 10,413
Cited by
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Leijtens, T., Bush, K. A., Prasanna, R., & McGehee, M. D. (2018) · Nature Energy · doi:10.1038/s41560-018-0190-4 · Cited by 1,121
Scalable fabrication and coating methods for perovskite solar cells and solar modules
Park, N.-G., & Zhu, K. (2020) · Nature Reviews Materials · doi:10.1038/s41578-019-0176-2 · Cited by 908
Synthetic Approaches for Halide Perovskite Thin Films
Dunlap-Shohl, W. A., Zhou, Y., Padture, N. P., & Mitzi, D. B. (2019) · Chemical Reviews · doi:10.1021/acs.chemrev.8b00318 · Cited by 631
Progress on Perovskite Materials and Solar Cells with Mixed Cations and Halide Anions
Ono, L. K., Juarez-Perez, E. J., & Qi, Y. (2017) · ACS Applied Materials & Interfaces · doi:10.1021/acsami.7b06001 · Cited by 593
Jošt, M., Kegelmann, L., Korte, L., & Albrecht, S. (2020) · Advanced Energy Materials · doi:10.1002/aenm.201904102 · Cited by 538
Metadata
- Authors
- Momblona, C., Gil-Escrig, L., Bandiello, E., Hutter, E. M., Sessolo, M., Lederer, K., Blochwitz-Nimoth, J., & Bolink, H. J.
- Venue
- Energy Environ. Sci.
- Publisher
- Royal Society of Chemistry (RSC)
- Published
- 2016
- Volume
- 9
- Issue
- 11
- Pages
- 3456-3463
- ISSN
- 1754-5692 (ISSN-L)
- 1754-5706
- OpenAlex
- W2523573243
- Cited by
- 514
- References
- 1
- FWCI
- 27.44
- Type
- journal article
- Language
- en
- Open access
- green
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- Momblona, C., Gil-Escrig, L., Bandiello, E., Hutter, E. M., Sessolo, M., Lederer, K., Blochwitz-Nimoth, J., & Bolink, H. J. (2016). Efficient vacuum deposited p-i-n and n-i-p perovskite solar cells employing doped charge transport layers. Energy Environ. Sci. https://doi.org/10.1039/c6ee02100j
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