Is the rapid initial performance loss of Fe/N/C non precious metal catalysts due to micropore flooding?
Abstract
The instability of Fe/N/C non-precious metal catalysts is still not fully understood, and must be overcome before these catalysts can be commercialized.
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PGM-free catalysts degrade severely during PEM fuel cell operation, which presents the primary bottleneck for deploying PGM-free catalysts.
“Importantly, PGM-free catalysts degrade severely during PEM fuel cell operation, which presents the primary bottleneck for deploying PGM-free catalysts [60,241].”
From Recent Advances on PEM Fuel Cells: From Key Materials to Membrane Electrode Assembly (2023) · cites this paper as [241]
Cites
High-Performance Electrocatalysts for Oxygen Reduction Derived from Polyaniline, Iron, and Cobalt
Wu, G., More, K. L., Johnston, C. M., & Zelenay, P. (2011) · Science · doi:10.1126/science.1200832 · Cited by 3,984 · see citing works
Uchida, M., Fukuoka, Y., Sugawara, Y., Eda, N., & Ohta, A. (1996) · Journal of The Electrochemical Society · doi:10.1149/1.1836988 · Cited by 309 · see citing works
Bimodal, templated mesoporous carbons for capacitor applications
Banham, D., Feng, F., Burt, J., Alsrayheen, E., & Birss, V. (2010) · Carbon · doi:10.1016/j.carbon.2009.11.025 · Cited by 56 · see citing works
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Wang, X. X., Swihart, M. T., & Wu, G. (2019) · Nature Catalysis · doi:10.1038/s41929-019-0304-9 · Cited by 1,174 · see citing works
Recent Advances on PEM Fuel Cells: From Key Materials to Membrane Electrode Assembly
Mo, S., Du, L., Huang, Z., Chen, J., Zhou, Y., Wu, P., Meng, L., Wang, N., Xing, L., Zhao, M., et al. (2023) · Electrochemical Energy Reviews · doi:10.1007/s41918-023-00190-w · Cited by 277 · see citing works
“Importantly, PGM-free catalysts degrade severely during PEM fuel cell operation, which presents the primary bottleneck for deploying PGM-free catalysts [60, 241].”
Self-citationExploring Durable Single-Atom Catalysts for Proton Exchange Membrane Fuel Cells
Wan, X., & Shui, J. (2022) · ACS Energy Letters · doi:10.1021/acsenergylett.2c00473 · Cited by 128 · see citing works
Ultralow platinum loading proton exchange membrane fuel cells: Performance losses and solutions
Banham, D., Zou, J., Mukerjee, S., Liu, Z., Yang, D., Zhang, Y., Peng, Y., & Dong, A. (2021) · Journal of Power Sources · doi:10.1016/j.jpowsour.2021.229515 · Cited by 103 · see citing works
Self-citation
- Authors
- Choi, J.-Y., Yang, L., Kishimoto, T., Fu, X., Ye, S., Chen, Z., & Banham, D.
- Affiliations
- University of Waterloo (CA)
- Ballard Power Systems (Canada) (CA)
- Nisshinbo Holdings (Japan) (JP)
- Corresponding author
- Chen, Zhongwei
- Banham, Dustin
- Venue
- Energy & Environmental Science
- Publisher
- Royal Society of Chemistry (RSC)
- Published
- 2017
- Volume
- 10
- Issue
- 1
- Pages
- 296-305
- ISSN
- 1754-5692 (ISSN-L)
- 1754-5706
- OpenAlex
- W2560726463
- Cited by
- 162
- References
- 3
- Citations by year
- 2026: 6 · 2025: 14 · 2024: 13 · 2023: 22 · 2022: 10 · 2021: 26 · 2020: 27 · 2019: 25 · 2018: 13 · 2017: 6
- FWCI
- 3.98
- Type
- journal article
- Language
- en
- Open access
- closed
- Locations
- Energy & Environmental Science (publishedVersion)
- Funders
- Simon Fraser University
- Natural Sciences and Engineering Research Council of Canada
- Topics
- Physical Sciences › Energy › Renewable Energy, Sustainability and the Environment › Electrocatalysts for Energy Conversion
- Physical Sciences › Engineering › Electrical and Electronic Engineering › Fuel Cells and Related Materials
- Physical Sciences › Materials Science › Materials Chemistry › Catalytic Processes in Materials Science
- Keywords
- Fe-N-C catalysts, non-precious metal electrocatalysts, oxygen reduction reaction, catalyst deactivation, catalyst stability
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