A ph, glucose, and dopamine triple-responsive, self-healable adhesive hydrogel formed by phenylborate-catechol complexation
Abstract
A pH, glucose, and dopamine triple-responsive, self-healable and adhesive polyethylene glycol hydrogel was developed via the formation of phenylborate–catechol complexation.
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Shan and coworkers developed a mussel-inspired PEG-based hydrogel containing catechol-modified four-armed PEG (4-arm-PEG-DA) and phenylboronic acid-functionalized four-armed PEG (4-arm-PEG-PBA); at pH 9.0, mixing the two modified PEGs led to the fast formation of a PEG-based hydrogel by boron ester-based crosslinking.
“For example, Shan and coworkers developed a mussel-inspired polyethylene glycol (PEG)-based hydrogel. The hydrogel contained catechol-modified four-armed PEG (4-arm-PEG-DA) and phenylboronic acid-functionalized four-armed PEG (4-arm-PEG-PBA). At pH 9.0, mixing the two modified PEGs led to the fast formation of a PEG-based hydrogel by boron ester-based crosslinking (borate–catechol complexation) [”
From Mussel-Inspired Injectable Adhesive Hydrogels for Biomedical Applications (2024) · cites this paper as [69]
Cites
Cross-Linking in Adhesive Quinoproteins: Studies with Model Decapeptides
Burzio, L. A., & Waite, J. H. (2000) · Biochemistry · doi:10.1021/bi0002434 · Cited by 485 · see citing works
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Recent progress in synthesis and application of mussel-inspired adhesives
Guo, Q., Chen, J., Wang, J., Zeng, H., & Yu, J. (2020) · Nanoscale · doi:10.1039/c9nr09780e · Cited by 370 · see citing works
Mussel-Inspired Injectable Adhesive Hydrogels for Biomedical Applications
Dou, W., Zeng, X., Zhu, S., Zhu, Y., Liu, H., & Li, S. (2024) · International Journal of Molecular Sciences · doi:10.3390/ijms25169100 · Cited by 52 · see citing works
“At pH 9.0, mixing the two modified PEGs led to the fast formation of a PEG-based hydrogel by boron ester-based crosslinking (borate–catechol complexation) [69].”
BackgroundInfluential
- Authors
- Shan, M., Gong, C., Li, B., & Wu, G.
- Affiliations
- Nankai University (CN)
- Corresponding author
- Wu, Guolin
- Venue
- Polymer Chemistry
- Publisher
- Royal Society of Chemistry (RSC)
- Published
- 2017
- Volume
- 8
- Issue
- 19
- Pages
- 2997-3005
- ISSN
- 1759-9954 (ISSN-L)
- 1759-9962
- OpenAlex
- W2607319610
- Cited by
- 151
- References
- 1
- Citations by year
- 2026: 7 · 2025: 12 · 2024: 25 · 2023: 15 · 2022: 19 · 2021: 19 · 2020: 20 · 2019: 16 · 2018: 12 · 2017: 6
- FWCI
- 5.68
- Type
- journal article
- Language
- en
- Open access
- closed
- Locations
- Polymer Chemistry (publishedVersion)
- Funders
- Natural Science Foundation of Tianjin City (14JCYBJC18100)
- National Natural Science Foundation of China (51203079)
- Topics
- Life Sciences › Biochemistry, Genetics and Molecular Biology › Molecular Medicine › Hydrogels: synthesis, properties, applications
- Physical Sciences › Materials Science › Polymers and Plastics › Polymer composites and self-healing
- Physical Sciences › Materials Science › Surfaces, Coatings and Films › Polymer Surface Interaction Studies
- Keywords
- self-healing hydrogels, adhesive hydrogels, pH-responsive, polyethylene glycol, stimuli-responsive materials
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