Cited by 60Organic Electronics and PhotovoltaicsPorphyrin and Phthalocyanine ChemistryPhotodynamic Therapy Research Studies

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Artificial light-harvesting n-type porphyrin for panchromatic organic photovoltaic devices

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Hadmojo, Wisnu Tantyo, Yim, Dajeong, Aqoma, Havid, Ryu, Du Yeol, Shin, Tae Joo, Kim, Hyun Woo, Hwang, Eojin, Jang, Woo-Dong, Jung, In Hwan, Jang, Sung-Yeon·2017·Chemical Science

DOI 10.1039/c7sc01275fPMC PMC5613227

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Abstract

We developed a novel NIR-harvesting n-type porphyrin derivative, PDI–P Zn –PDI, that shows a low bandgap of 1.27 eV. Panchromatic absorption was extended to the NIR area with a significantly low energy loss of 0.54 eV which led to promising photovoltaic performance.

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Scheme 1 Synthesis of PDI–PZn–PDI.CC BY · PubMed Central

Fig. 1 (a) UV-vis-NIR absorption spectra of PDI–PZn–PDI, PTB7-Th and PTB7-Th:PDI–PZn–PDI BHJ films (with or without pyridine). The cyan line indicates the EQE of the BHJ OPV devices. (b) CV results of PDI–PZn–PDI and PTB7-Th. (c) Band diagrams of PDI–PZn–PDI and PTB7-Th determined from electrochemical (lines) and optical (boxes) analyses.CC BY · PubMed Central

Fig. 2 Geometric structures of PDI–PZn–PDI calculated by the DFT method using B3LYP/6-31G(d, p). (a) HOMO and LUMO of PDI–PZn–PDI, (b) side view of the tube shape, with and without pyridine, and (c) charge variation from the ground state (S0) to the excited state (S1).CC BY · PubMed Central

Fig. 3 (a) The J–V characteristics of inverted-structure BHJ OPV devices (the inset shows the device architecture); (b) EQE of the PTB7-Th:PDI–PZn–PDI photovoltaic devices corresponding to the J SC values.CC BY · PubMed Central

Fig. 4 2D-GIXD images of pristine and blend films: (a) PTB7-Th, (b) PDI–PZn–PDI and (c) PTB7-Th : PDI–PZn–PDI (1.0 : 1.2 w/w) without pyridine, and (e) PTB7-Th, (f) PDI–PZn–PDI and (g) PTB7-Th : PDI–PZn–PDI (1.0 : 1.2 w/w) with 0.8 vol% pyridine. Inset images are the corresponding AFM images. TEM images of PTB7-Th : PDI–PZn–PDI (1.0 : 1.2 w/w) (d) without or (h) with pyridine. (i) Out-of-plane and in-plane line-cut of the PDI–PZn–PDI film with or without pyridine and (j) PDI–PZn–PDI ordering with pyridine.CC BY · PubMed Central

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Authors: Hadmojo, W. T., Yim, D., Aqoma, H., Ryu, D. Y., Shin, T. J., Kim, H. W., Hwang, E., Jang, W.-D., Jung, I. H., & Jang, S.-Y.
Affiliations: Kookmin University (KR)
Yonsei University (KR)
Ulsan National Institute of Science and Technology (KR)
Korea Research Institute of Chemical Technology (KR)
Corresponding author: Jang, Woo-Dong
Jung, In Hwan
Jang, Sung-Yeon
ORCID: Hadmojo, Wisnu Tantyo
Aqoma, Havid
Ryu, Du Yeol
Shin, Tae Joo
Kim, Hyun Woo
Jang, Woo-Dong
Jung, In Hwan
Jang, Sung-Yeon
Venue: Chemical Science
Publisher: Royal Society of Chemistry (RSC)
Published: 2017
Volume: 8
Issue: 7
Pages: 5095-5100
ISSN: 2041-6520 (ISSN-L)
2041-6539
DOI: 10.1039/c7sc01275f
PMC: PMC5613227
OpenAlex: W2615045677
Cited by: 60
References: 37
Citations by year: 2026: 3 · 2025: 3 · 2024: 4 · 2023: 5 · 2022: 4 · 2021: 6 · 2020: 7 · 2019: 10 · 2018: 13 · 2017: 5
FWCI: 3.98
Type: journal article
Language: en
Open access: diamond
doi.org
Licence: cc-by
Locations: Chemical Science (publishedVersion, cc-by)
PubMed Central (publishedVersion, cc-by)
PubMed (publishedVersion)
Scholarworks@UNIST (Ulsan National Institute of Science and Technology) (submittedVersion)
Funders: National Research Foundation of Korea (2016M1A2A2940912, 2016R1A5A1012966, 2017R1C1B2010694, 2014R1A2A1A10051083)
Korea Institute of Energy Technology Evaluation and Planning (20163030013960)
Topics: Physical Sciences › Engineering › Electrical and Electronic Engineering › Organic Electronics and Photovoltaics
Physical Sciences › Materials Science › Materials Chemistry › Porphyrin and Phthalocyanine Chemistry
Life Sciences › Biochemistry, Genetics and Molecular Biology › Cancer Research › Photodynamic Therapy Research Studies
Keywords: zinc porphyrin, artificial light harvesting, panchromatic absorption, near-infrared absorption, organic solar cells, low band gap, energy loss

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Artificial light-harvesting n-type porphyrin for panchromatic organic photovoltaic devices

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