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Cited by 292Catalysis for Biomass Conversionbiodegradable polymer synthesis and propertiesBiofuel production and bioconversion

Advances in catalytic routes for the production of carboxylic acids from biomass: A step forward for sustainable polymers

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Iglesias, J., Martínez-Salazar, I., Maireles-Torres, P., Martin Alonso, D., Mariscal, R., López Granados, M.·2020·Chemical Society Reviews
DOI 10.1039/d0cs00177e
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Abstract

Polymers are ubiquitously present in our daily life because they can meet a wide range of needs and fields of applications. This success, based on an irresponsible linear consumption of plastics and the access to cheap oil, is creating serious environmental problems. Two lines of actions are needed to cope with them: to adopt a circular consumption of plastics and to produce renewable carbon-neutral monomers. This review analyses the recent advances in the chemocatalytic processes for producing biomass-derived carboxylic acids. These renewable carboxylic acids are involved in the synthesis of relevant general purpose and specialty polyesters and polyamides; some of them are currently derived from oil, while others can become surrogates of petrochemical polymers due to their excellent performance properties. Polyesters and polyamides are very suitable to be depolymerised to other valuable chemicals or to their constituent monomers, what facilitates the circular reutilisation of these monomers. Different types of carboxylic acids have been included in this review: monocarboxylic acids (like glycolic, lactic, hydroxypropanoic, methyl vinyl glycolic, methyl-4-methoxy-2-hydroxybutanoic, 2,5-dihydroxypent-3-enoic, 2,5,6-trihydroxyhex-3-enoic acids, diphenolic, acrylic and δ-amino levulinic acids), dicarboxylic acids (2,5-furandicarboxylic, maleic, succinic, adipic and terephthalic acids) and sugar acids (like gluconic and glucaric acids). The review evaluates the technology status and the advantages and drawbacks of each route in terms of feedstock, reaction pathways, catalysts and economic and environmental evaluation. The prospects and the new research that should be undertaken to overcome the main problems threatening their economic viability or the weaknesses that prevent their commercial implementation have also been underlined.

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  • Short chain fatty acids/volatile fatty acids are essential industrial chemicals used for the production of acidulant, flavoring agents, polymers, preservatives and many other applications in food, pharmaceutical, and cosmetic industries.

    “Short chain fatty acids/volatile fatty acids are essential industrial chemicals used for the production of acidulant, flavoring agents, polymers, preservatives and many other applications in food industry, pharmaceutical industries, and cosmetic industries [85,86].”

    From Food Waste Biorefinery: Pathway towards Circular Bioeconomy (2021) · cites this paper as [86]

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200 of 511 shown

Authors
Iglesias, J., Martínez-Salazar, I., Maireles-Torres, P., Martin Alonso, D., Mariscal, R., & López Granados, M.
Affiliations
  • Universidad Rey Juan Carlos (ES)
  • Consejo Superior de Investigaciones Científicas (ES)
  • Universidad de Málaga
  • Glucan Biorenewables LLC
  • EQS Group (Sustainable Energy and Chemistry Group)
ORCID
Venue
Chemical Society Reviews
Publisher
Royal Society of Chemistry (RSC)
Published
2020
Volume
49
Issue
16
Pages
5704-5771
ISSN
  • 0306-0012 (ISSN-L)
  • 1460-4744
DOI
10.1039/d0cs00177e
OpenAlex
W3041663202
Cited by
292
References
529
Citations by year
2026: 43 · 2025: 59 · 2024: 64 · 2023: 38 · 2022: 46 · 2021: 36 · 2020: 6
FWCI
2.63
Type
journal article
Language
en
Open access
Licence
Locations
  • Chemical Society Reviews (publishedVersion, cc-by-nc)
  • PubMed (publishedVersion)
  • DIGITAL.CSIC (Spanish National Research Council (CSIC)) (acceptedVersion)
  • BURJC Digital (King Juan Carlos University) (submittedVersion, cc-by-nc)
  • Hispana (submittedVersion, cc-by-nc)
Funders
  • Ministerio de Ciencia e Innovación (RTI2018-094918-B-C41, RTI2018-094918-B-C42, RTI2018-094918-B-C44)
  • Comunidad de Madrid (S2018/EMT-4344 (BIOTRES-CM))
  • European Regional Development Fund (S2018/EMT-4344 (BIOTRES-CM))
Topics
  • Physical Sciences › Engineering › Biomedical Engineering › Catalysis for Biomass Conversion
  • Physical Sciences › Materials Science › Biomaterials › biodegradable polymer synthesis and properties
  • Physical Sciences › Engineering › Biomedical Engineering › Biofuel production and bioconversion
Keywords
chemocatalysis, renewable monomers, polyester synthesis, polyamide synthesis, circular economy, 2,5-furandicarboxylic acid, succinic acid, adipic acid, terephthalic acid, maleic acid, levulinic acid, glycolic acid, lactic acid, gluconic acid, glucaric acid, sugar acids, catalysts, economic and environmental evaluation

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