A sub-ppm upper limit on the cosmological variations of the fine structure constant α
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Abstract
Absorption spectroscopy toward high-redshift quasars provides strong constraints on the putative variation of fundamental constants of physics on cosmological timescales. The submillimeter ground-state transitions of methylidyne (CH) and water (H 2 O), both molecules widespread and coeval in the interstellar medium, provide a sensitive test for variations in α , the fine structure constant, and μ , the proton-to-electron mass ratio, taking advantage of the unmatched spectral resolution and frequency reliability of radio techniques. We used ALMA simultaneous observations of the two species to constrain any velocity offset between their absorption profiles toward the radio-bright lensed quasars PKS 1830−211 ( z abs = 0.89) and B 0218+357 ( z abs = 0.68). Our observational setup minimizes instrumental errors and known sources of systematics, such as time variability of the absorption profile and frequency-dependent morphology of the background quasar. The excellent correlation between CH and H 2 O opacities, the large number of individual narrow velocity components, and the number of independent spectra obtained due to the intrinsic time variability of the absorption profiles ensure that even the chemical segregation bias is minimized. We obtained bulk velocity shifts of δv = −0.048 ± 0.028 km s −1 and −0.13 ± 0.14 km s −1 (1 σ confidence level) between CH and H 2 O in the direction of PKS 1830−211(NE) and B 0218+357(SW), respectively. These values convert into the 3 σ upper limits |Δ α / α |< 0.55 ppm and 1.5 ppm, respectively, taking into account the independent upper limits on |Δ μ / μ | previously obtained for these systems. These constraints on |Δ α / α |, at look-back times of about half the present age of the Universe, are two to four times deeper than previous constraints on any other single high- z system.
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ALMA measurements of absorption spectroscopy toward high-redshift quasars bound the variation Δα = α(z=0.89)-α0 to |Δα/α0| < 0.55 p.p.m.
“ALMA measurements of absorption spectroscopy toward high-redshift quasars bound the variation ∆α = α(z = 0.89)-α 0 to |∆α/α 0 | < 0.55p.p.m [14] [15,16].”
From Stress-energy tensor of a scalar field on a product spacetime with a time-dependent compact dimension (2026) · cites this paper as [14]
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Search for Time Variation of the Fine Structure Constant
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Further evidence for a variable fine-structure constant from Keck/HIRES QSO absorption spectra
Murphy, M. T., Webb, J. K., & Flambaum, V. V. (2003) · Monthly Notices of the Royal Astronomical Society · doi:10.1046/j.1365-8711.2003.06970.x · Cited by 514 · see citing works
Self-citationIndications of a Spatial Variation of the Fine Structure Constant
Webb, J. K., King, J. A., Murphy, M. T., Flambaum, V. V., Carswell, R. F., & Bainbridge, M. B. (2011) · Physical Review Letters · doi:10.1103/physrevlett.107.191101 · Cited by 482 · see citing works
Self-citationHart, L., & Chluba, J. (2020) · Monthly Notices of the Royal Astronomical Society · doi:10.1093/mnras/staa412 · Cited by 130 · see citing works
Molaro, P., Centurión, M., Whitmore, J. B., Evans, T. M., Murphy, M. T., Agafonova, I. I., Bonifacio, P., D’Odorico, S., Levshakov, S. A., Lopez, S., et al. (2013) · Astronomy & Astrophysics · doi:10.1051/0004-6361/201321351 · Cited by 111 · see citing works
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Self-citationImpact of instrumental systematic errors on fine-structure constant measurements with quasar spectra
Whitmore, J. B., & Murphy, M. T. (2014) · Monthly Notices of the Royal Astronomical Society · doi:10.1093/mnras/stu2420 · Cited by 99 · see citing works
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Self-citationThe mystery of alpha and the isotopes
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Research works printed but not linked: 2
- Mahieu, S., Maier, D., Lazareff, B., et al., 2012, IEEE Trans. Terahertz Sci. Technol., 2, 29
- Sch¨ oneberg, N. & Vacher, L., 2025, Journal of Cosmology and Astroparticle Physics, 03, 004
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Paul, A., & Paban, S. (2026) · Journal of High Energy Physics · doi:10.1007/jhep09(2026)188
- Authors
- Muller, S., Beelen, A., Guélin, M., Black, J. H., Combes, F., Bethlem, H. L., Gérin, M., Henkel, C., Menten, K. M., Murphy, M. T., Ubachs, W., & Wozny, N.
- Affiliations
- Department of Space, Earth and Environment, Chalmers University of Technology, Onsala Space Observatory
- Centre National de la Recherche Scientifique (FR)
- Chalmers University of Technology (SE)
- Vrije Universiteit Amsterdam (NL)
- Max Planck Society (DE)
- Swinburne University of Technology (AU)
- ORCID
- Venue
- Astronomy & Astrophysics
- Publisher
- EDP Sciences
- Published
- 2026-02
- Volume
- 706
- Pages
- A365
- ISSN
- 0004-6361 (ISSN-L)
- 1432-0746
- OpenAlex
- W4417469605
- Cited by
- 3
- References
- 10
- Citations by year
- 2026: 3
- FWCI
- 9.24
- Type
- journal article
- Language
- en
- Open access
- gold
- doi.org
- Licence
- Locations
- Astronomy and Astrophysics (publishedVersion, cc-by)
- VU Research Portal (publishedVersion, cc-by)
- HAL AMU (submittedVersion)
- arXiv (Cornell University) (submittedVersion)
- Chalmers Research (Chalmers University of Technology) (submittedVersion)
- DOAJ (DOAJ: Directory of Open Access Journals) (submittedVersion)
- arXiv (Cornell University)
- Funders
- National Science Foundation
- National Aeronautics and Space Administration
- National Radio Astronomy Observatory
- National Science Council
- National Astronomical Observatory of Japan
- National Institutes of Natural Sciences
- Topics
- Physical Sciences › Physics and Astronomy › Astronomy and Astrophysics › Cosmology and Gravitation Theories
- Physical Sciences › Physics and Astronomy › Astronomy and Astrophysics › Astrophysics and Star Formation Studies
- Physical Sciences › Physics and Astronomy › Astronomy and Astrophysics › Stellar, planetary, and galactic studies
- Keywords
- fine-structure constant variation, proton-electron mass ratio, interstellar absorption, high-redshift quasars, PKS 1830-211, B0218+357, lensed quasars, ALMA, fundamental physical constants
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