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Fluorescence quantum yield of CdSe/ZnS nanocrystals investigated by correlated atomic-force and single-particle fluorescence microscopy
Abstract
Correlated atomic-force and fluorescence microscopy are used to study single-particle versus ensemble fluorescence quantum yields (QY) of semiconductor nanocrystals by measuring a simultaneous map of the topography and the single-particle fluorescence. CdSe/ZnS nanocrystal quantum dots and quantum rods with high QY were investigated. A significant portion of dark particles is detected. Comparison with the ensemble solution QY shows that samples with higher QY have a larger fraction of bright particles accompanied by an increased single-particle QY. Saturated emission from single nanocrystals could not be detected because of particle darkening under high-power excitation.
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Cites
Shape control of CdSe nanocrystals
Peng, X., Manna, L., Yang, W., Wickham, J., Scher, E., Kadavanich, A., & Alivisatos, A. P. (2000) · Nature · doi:10.1038/35003535 · Cited by 4,487
Dabbousi, B. O., Rodriguez-Viejo, J., Mikulec, F. V., Heine, J. R., Mattoussi, H., Ober, R., Jensen, K. F., & Bawendi, M. G. (1997) · The Journal of Physical Chemistry B · doi:10.1021/jp971091y · Cited by 4,229
Cited by
Quantum Dots and Their Multimodal Applications: A Review
Bera, D., Qian, L., Tseng, T.-K., & Holloway, P. H. (2010) · Materials · doi:10.3390/ma3042260 · Cited by 1,365
de Mello Donegá, C., Liljeroth, P., & Vanmaekelbergh, D. (2005) · Small · doi:10.1002/smll.200500239 · Cited by 511
Mekis, I., Talapin, D. V., Kornowski, A., Haase, M., & Weller, H. (2003) · The Journal of Physical Chemistry B · doi:10.1021/jp0278364 · Cited by 375
Metadata
- Authors
- Ebenstein, Y., Mokari, T., & Banin, U.
- Venue
- Applied Physics Letters
- Publisher
- AIP Publishing
- Published
- 2002-05-27
- Volume
- 80
- Issue
- 21
- Pages
- 4033-4035
- ISSN
- 0003-6951 (ISSN-L)
- 1077-3118
- OpenAlex
- W2026632985
- Cited by
- 216
- References
- 2
- FWCI
- 9.12
- Type
- journal article
- Language
- en
- Open access
- closed
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- Ebenstein, Y., Mokari, T., & Banin, U. (2002). Fluorescence quantum yield of CdSe/ZnS nanocrystals investigated by correlated atomic-force and single-particle fluorescence microscopy. Applied Physics Letters. https://doi.org/10.1063/1.1482785
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