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Nucleation and growth kinetics of nanocrystals formed upon pulsed-laser ablation in liquid
Abstract
To have a clear physical insight into the nanocrystal formation upon pulsed-laser ablation in liquid, we proposed a theoretical kinetic approach to elucidate the nucleation and growth of nanocrystals with respect to the capillary effect of the nanometer-sized curvature of crystalline nuclei. Taking the nanodiamond synthesis by pulsed-laser ablating a graphite target in water as an example, we predicted the nucleation time, growth velocity, and the grown size of nanodiamonds on the basis of the proposed kinetic model, and found that these theoretical results are in well agreement with our experiment cases. We expected that the kinetic approach is generally applicable to understanding the basic physics of nanocrystal formation in pulsed-laser ablation in liquid.
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“Wang et al. [91] proposed a theoretical kinetic approach and validated with experimental work that the isothermal nucleation time ranges between 10−10 second and 1 nanosecond.”
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Metadata
- Authors
- Wang, C. X., Liu, P., Cui, H., & Yang, G. W.
- Affiliations
- State Key Laboratory of Optoelectronic Materials and Technology (CN)
- Venue
- Applied Physics Letters
- Publisher
- AIP Publishing
- Published
- 2005-11-10
- Volume
- 87
- Issue
- 20
- ISSN
- 0003-6951 (ISSN-L)
- 1077-3118
- OpenAlex
- W1966655708
- Cited by
- 113
- References
- 25
- Citations by year
- 2025: 1 · 2024: 3 · 2023: 3 · 2022: 4 · 2021: 5 · 2020: 6 · 2019: 2 · 2018: 5 · 2017: 4 · 2016: 9 · 2015: 3 · 2014: 10 · 2013: 10 · 2012: 7
- FWCI
- 3.70
- Type
- journal article
- Language
- en
- Open access
- closed
- Locations
- Applied Physics Letters (publishedVersion)
- Topics
- Physical Sciences › Materials Science › Materials Chemistry › Laser-Ablation Synthesis of Nanoparticles
- Physical Sciences › Physics and Astronomy › Acoustics and Ultrasonics › Ultrasound and Cavitation Phenomena
- Physical Sciences › Materials Science › Materials Chemistry › Diamond and Carbon-based Materials Research
- Keywords
- pulsed laser ablation in liquid, nanocrystal nucleation, nanocrystal growth kinetics, nanodiamond synthesis, capillarity, graphite target, growth rate (crystal and thin-film growth), nucleation time, kinetic model
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