Influence of Water Temperature on the Hydrodynamic Diameter of Gold Nanoparticles from Laser Ablation
Abstract
Defined hydrodynamic properties of nanoparticle colloids are required for applications in dosimetry, rheology, or biosensing studies. During the generation of nanoparticles by laser ablation of a solid target in liquids, the temperature of the liquid increases, which may effect cavitation bubble and particle formation. We demonstrate that this temperature variation influences the hydrodynamic diameter of the resulting colloidal nanoparticles when a gold target is ablated by an IR femtosecond laser in water at different stabilized liquid temperatures in the range of 283−353 K. The maximum hydrodynamic diameter was observed at 330 K, the temperature at which the compressibility of water reaches its minimum. The formation of particles by condensation of ablated species in the liquid matrix or inside the confined cavitation bubble is discussed, as well as the influence of the physical properties of the liquid that vary with temperature, such as viscosity and compressibility. The reduction of the hydrodynamic particle diameter at the higher compressible state of water indicates that a lower number of agglomerates are dispersed in the liquid, reducing the polydispersity index of the gold colloid.
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Menendez et al. concluded that due to a reduction in the hydrodynamic particle diameter, few agglomerates are dispersed in the liquid, thereby reducing the poly-dispersity index of Au NPs.
“They concluded that due to a reduction in the hydrodynamic particle diameter, few agglomerates are dispersed in the liquid, thereby reducing the poly-dispersity index of Au NPs.”
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Upscaling Pulsed Laser Fragmentation in Liquids by Advanced Free‐Flow Setups
Kricke, J. L., Fu, Z., Burgmann, S., Janoske, U., Doñate‐Buendía, C., & Gökce, B. (2026) · Advanced Materials Technologies · doi:10.1002/admt.71236
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- Authors
- Menéndez-Manjón, A., Chichkov, B. N., & Barcikowski, S.
- Affiliations
- Laser Zentrum Hannover (DE)
- Corresponding author
- Barcikowski, Stephan
- Venue
- The Journal of Physical Chemistry C
- Publisher
- American Chemical Society (ACS)
- Published
- 2010-01-22
- Volume
- 114
- Issue
- 6
- Pages
- 2499-2504
- ISSN
- 1932-7447 (ISSN-L)
- 1932-7455
- OpenAlex
- W2095031846
- Cited by
- 79
- References
- 34
- Citations by year
- 2026: 6 · 2025: 3 · 2024: 8 · 2023: 7 · 2022: 3 · 2021: 2 · 2020: 5 · 2019: 3 · 2018: 2 · 2017: 6 · 2016: 4 · 2015: 6 · 2014: 1 · 2013: 5 · 2012: 10
- FWCI
- 4.34
- Type
- journal article
- Language
- en
- Open access
- closed
- Locations
- The Journal of Physical Chemistry C (publishedVersion)
- Topics
- Physical Sciences › Engineering › Biomedical Engineering › Laser-Ablation Synthesis of Nanoparticles
- Physical Sciences › Materials Science › Electronic, Optical and Magnetic Materials › Gold and Silver Nanoparticles Synthesis and Applications
- Physical Sciences › Materials Science › Materials Chemistry › Ultrasound and Cavitation Phenomena
- Keywords
- gold nanoparticles, hydrodynamic diameter, laser ablation in liquid, water temperature, cavitation bubbles, femtosecond laser ablation, water compressibility, nanoparticle agglomeration, polydispersity index, colloidal nanoparticles, viscosity
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