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A systematic analysis of the spectra of the lanthanides doped into single crystal LaF3
Abstract
The optical spectra of the lanthanides doped into single crystal LaF3 have been interpreted in terms of transitions within 4f N configurations. Energy matrices combining free-ion terms with a crystal field for an approximate model which assumes C2v instead of the actual C2 site symmetry were diagonalized. Excellent correlations were obtained between experimental transition energies and the computed level structures. We also report the results of previously unpublished experimental spectroscopic investigations of Nd3+ and Sm3+:LaF3, as well as predicted energy levels for Pm3+:LaF3. The spectroscopic data for each ion were independently interpreted using an effective-operator model, then the model parameters were intercompared. Systematic trends have been identified, and a comprehensive energy level diagram is presented.
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Citations
Cites
Theory of lanthanide crystal fields
Newman, D. J. (1971) · Advances in Physics · doi:10.1080/00018737100101241 · Cited by 689
Cited by
Zheng, W., Huang, P., Tu, D., Ma, E., Zhu, H., & Chen, X. (2015) · Chemical Society Reviews · doi:10.1039/c4cs00178h · Cited by 894
Optical temperature sensing of up-conversion luminescent materials: Fundamentals and progress
Zhao, Y., Wang, X., Zhang, Y., Li, Y., & Yao, X. (2020) · Journal of Alloys and Compounds · doi:10.1016/j.jallcom.2019.152691 · Cited by 380
Metadata
- Authors
- Carnall, W. T., Goodman, G. L., Rajnak, K., & Rana, R. S.
- Venue
- The Journal of Chemical Physics
- Publisher
- AIP Publishing
- Published
- 1989-04-01
- Volume
- 90
- Issue
- 7
- Pages
- 3443-3457
- ISSN
- 0021-9606 (ISSN-L)
- 1089-7690
- OpenAlex
- W2127119100
- Cited by
- 1,239
- References
- 1
- FWCI
- 21.11
- Type
- journal article
- Language
- en
- Open access
- closed
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- CoChat. (2026). Citation check: A systematic analysis of the spectra of the lanthanides doped into single crystal LaF3. https://app.cochat.ai/papers/10.1063/1.455853
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- Carnall, W. T., Goodman, G. L., Rajnak, K., & Rana, R. S. (1989). A systematic analysis of the spectra of the lanthanides doped into single crystal LaF3. The Journal of Chemical Physics. https://doi.org/10.1063/1.455853
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