Cited by 22Magnetic properties of thin filmsLaser-Matter Interactions and ApplicationsMultiferroics and related materials

Femtosecond photocurrents at the FeRh/Pt interface

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Medapalli, R., Li, G., Patel, Sheena K. K., Mikhaylovskiy, R. V., Rasing, Th., Kimel, A. V., Fullerton, E. E.·2020·Applied Physics Letters

Abstract

Femtosecond laser excitations of FeRh/Pt bilayers launch an ultrafast pulse of electric photocurrents in the Pt-layer and subsequently result in the emission of electromagnetic radiation in the THz spectral range. Analysis of the THz emission as a function of the polarization of the femtosecond laser pulse, external magnetic field, sample temperature, and sample orientation shows that the photocurrent can emerge due to vertical spin pumping and photo-induced inverse spin–orbit torque at the FeRh/Pt interface. The vertical spin pumping from FeRh into Pt does not depend on the polarization of light and originates from ultrafast laser-induced demagnetization of the ferromagnetic phase of FeRh. The photo-induced inverse spin–orbit torque at the FeRh/Pt interface can be described in terms of a helicity-dependent effect of circularly polarized light on the magnetization of the ferromagnetic FeRh and the subsequent generation of a photocurrent.

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  • Similar THz emission has been observed in FeRh/Pt heterostructures and in FM/NM/NM heterostructures used in IREE investigations, but was conspicuously absent in FM/NM control devices.

    “Similar THz emission has been observed in FeRh/Pt heterostructures138 as well as the FM/NM/NM heterostructures used in investigations of the IREE, but were conspicuously absent in FM/NM control devices54.”

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Authors
Medapalli, R., Li, G., Patel, S. K. K., Mikhaylovskiy, R. V., Rasing, T., Kimel, A. V., & Fullerton, E. E.
Affiliations
  • University of California San Diego (US)
  • Radboud University Nijmegen (NL)
Corresponding author
Medapalli, R.
Venue
Applied Physics Letters
Published
2020-10-05
Volume
117
Issue
14
ISSN
  • 0003-6951 (ISSN-L)
  • 1077-3118
OpenAlex
W3092425042
Cited by
22
References
33
Citations by year
2026: 4 · 2025: 1 · 2024: 2 · 2023: 4 · 2022: 4 · 2021: 6 · 2020: 1
FWCI
1.53
Type
journal article
Language
en
Open access
Locations
  • Applied Physics Letters (publishedVersion)
  • Lancaster EPrints (Lancaster University) (submittedVersion)
  • OSTI OAI (U.S. Department of Energy Office of Scientific and Technical Information) (submittedVersion)
  • Radboud Repository (Radboud University) (submittedVersion)
  • Radboud Repository (Radboud University) (submittedVersion, other-oa)
Funders
  • U.S. Department of Energy (DE-SC0018237)
  • Nederlandse Organisatie voor Wetenschappelijk Onderzoek
Topics
  • Physical Sciences › Physics and Astronomy › Atomic and Molecular Physics, and Optics › Magnetic properties of thin films
  • Physical Sciences › Physics and Astronomy › Atomic and Molecular Physics, and Optics › Laser-Matter Interactions and Applications
  • Physical Sciences › Materials Science › Electronic, Optical and Magnetic Materials › Multiferroics and related materials
Keywords
terahertz emission, ultrafast demagnetization, ferromagnetic thin films, circularly polarized light, spintronics, laser-induced demagnetization

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