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Water-stable organic transistors and their application in chemical and biological sensors
Open accessAbstract
The development of low-cost, reliable sensors will rely on devices capable of converting an analyte binding event to an easily read electrical signal. Organic thin-film transistors (OTFTs) are ideal for inexpensive, single-use chemical or biological sensors because of their compatibility with flexible, large-area substrates, simple processing, and highly tunable active layer materials. We have fabricated low-operating voltage OTFTs with a cross-linked polymer gate dielectric, which display stable operation under aqueous conditions over >10 4 electrical cycles using the p-channel semiconductor 5,5′-bis-(7-dodecyl-9H-fluoren-2-yl)-2,2′-bithiophene (DDFTTF). OTFT sensors were demonstrated in aqueous solutions with concentrations as low as parts per billion for trinitrobenzene, methylphosphonic acid, cysteine, and glucose. This work demonstrates of reliable OTFT operation in aqueous media, hence opening new possibilities of chemical and biological sensing with OTFTs.
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Cites
Label-free immunodetection with CMOS-compatible semiconducting nanowires
Stern, E., Klemic, J. F., Routenberg, D. A., Wyrembak, P. N., Turner-Evans, D. B., Hamilton, A. D., LaVan, D. A., Fahmy, T. M., & Reed, M. A. (2007) · Nature · doi:10.1038/nature05498 · Cited by 1,352
Cited by
Highly sensitive flexible pressure sensors with microstructured rubber dielectric layers
Mannsfeld, S. C. B., Tee, B. C.-K., Stoltenberg, R. M., Chen, C. V. H.-H., Barman, S., Muir, B. V. O., Sokolov, A. N., Reese, C., & Bao, Z. (2010) · Nature Materials · doi:10.1038/nmat2834 · Cited by 3,291
Self-citationHammock, M. L., Chortos, A., Tee, B. C. ‐., Tok, J. B. ‐., & Bao, Z. (2013) · Advanced Materials · doi:10.1002/adma.201302240 · Cited by 2,396
Self-citationSchwartz, G., Tee, B. C.-K., Mei, J., Appleton, A. L., Kim, D. H., Wang, H., & Bao, Z. (2013) · Nature Communications · doi:10.1038/ncomms2832 · Cited by 2,042
Self-citationPan, L., Chortos, A., Yu, G., Wang, Y., Isaacson, S., Allen, R., Shi, Y., Dauskardt, R., & Bao, Z. (2014) · Nature Communications · doi:10.1038/ncomms4002 · Cited by 1,519
Self-citationQuinn, J. T. E., Zhu, J., Li, X., Wang, J., & Li, Y. (2017) · Journal of Materials Chemistry C · doi:10.1039/c7tc01680h · Cited by 452
Metadata
- Authors
- Roberts, M. E., Mannsfeld, S. C. B., Queraltó, N., Reese, C., Locklin, J., Knoll, W., & Bao, Z.
- Venue
- Proceedings of the National Academy of Sciences
- Published
- 2008-08-26
- Volume
- 105
- Issue
- 34
- Pages
- 12134-12139
- ISSN
- 0027-8424 (ISSN-L)
- 1091-6490
- OpenAlex
- W2024782002
- Cited by
- 358
- References
- 1
- FWCI
- 29.88
- Type
- journal article
- Language
- en
- Open access
- green
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- Roberts, M. E., Mannsfeld, S. C. B., Queraltó, N., Reese, C., Locklin, J., Knoll, W., & Bao, Z. (2008). Water-stable organic transistors and their application in chemical and biological sensors. Proceedings of the National Academy of Sciences. https://doi.org/10.1073/pnas.0802105105
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