Cited by 958Metal-Organic Frameworks: Synthesis and ApplicationsMembrane Separation and Gas TransportCarbon Dioxide Capture Technologies

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Metal-organic frameworks with high capacity and selectivity for harmful gases

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Britt, David, Tranchemontagne, David, Yaghi, Omar M.·2008·Proceedings of the National Academy of Sciences

DOI 10.1073/pnas.0804900105PMC PMC2575308

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Abstract

Benchmarks have been established for the performance of six metal-organic frameworks (MOFs) and isoreticular MOFs (IRMOFs, which have the same underlying topology as MOF-5), MOF-5, IRMOF-3, MOF-74, MOF-177, MOF-199, and IRMOF-62, as selective adsorbents for eight harmful gases: sulfur dioxide, ammonia, chlorine, tetrahydrothiophene, benzene, dichloromethane, ethylene oxide, and carbon monoxide. Kinetic breakthrough measurements are used to determine the calculated dynamic adsorption capacity of each “benchmark” MOF for each gas. The capacity of each MOF is compared to that of a sample of Calgon BPL activated carbon. We find that pore functionality plays a dominant role in determining the dynamic adsorption performance of MOFs. MOFs featuring reactive functionality outperform BPL carbon in all but one case and exhibit high dynamic adsorption capacities up to 35% by weight.

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D Tranchemontagne The Synthesis and Investigation of Alkyne-Containing Isoreticular Metal–Organic Frameworks for Hydrogen Storage and the Preliminary Investigation of Metal–Organic Frameworks for Gas Separation Applications. (Univ of California Los Angeles PhD thesis. (2007).

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Authors: Britt, D., Tranchemontagne, D., & Yaghi, O. M.
Affiliations: California NanoSystems Institute (US)
ORCID: Britt, David
Yaghi, Omar M.
Venue: Proceedings of the National Academy of Sciences
Publisher: National Academy of Sciences
Published: 2008-08-19
Volume: 105
Issue: 33
Pages: 11623-11627
ISSN: 0027-8424 (ISSN-L)
1091-6490
DOI: 10.1073/pnas.0804900105
PMC: PMC2575308
OpenAlex: W2116516840
Cited by: 958
References: 27
Citations by year: 2026: 34 · 2025: 34 · 2024: 55 · 2023: 47 · 2022: 60 · 2021: 79 · 2020: 62 · 2019: 64 · 2018: 78 · 2017: 48 · 2016: 57 · 2015: 61 · 2014: 46 · 2013: 60 · 2012: 51
FWCI: 24.47
Type: journal article
Language: en
Open access: green
www.ncbi.nlm.nih.gov
Locations: Proceedings of the National Academy of Sciences (publishedVersion)
PubMed Central (publishedVersion)
PubMed (publishedVersion)
Topics: Physical Sciences › Chemistry › Inorganic Chemistry › Metal-Organic Frameworks: Synthesis and Applications
Physical Sciences › Chemical Engineering › Filtration and Separation › Membrane Separation and Gas Transport
Physical Sciences › Chemical Engineering › Filtration and Separation › Carbon Dioxide Capture Technologies
Keywords: metal-organic frameworks, isoreticular MOFs, gas adsorption, dynamic adsorption capacity, harmful gas removal, sulfur dioxide, ammonia, chlorine, tetrahydrothiophene, benzene, dichloromethane, ethylene oxide, carbon monoxide, MOF-5, MOF-74, MOF-177, HKUST-1, IRMOF-3, activated carbon comparison
MeSH terms: Gases, Kinetics, Metals, Models, Molecular, Organic Chemicals, Molecular Structure, Crystallography, X-Ray

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Metal-organic frameworks with high capacity and selectivity for harmful gases

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