The DOI matches its Crossref record; 43 of the 43 references it cites were found in a registry or an index.
Imaging electronic quantum motion with light
Open accessAbstract
Imaging the quantum motion of electrons not only in real-time, but also in real-space is essential to understand for example bond breaking and formation in molecules, and charge migration in peptides and biological systems. Time-resolved imaging interrogates the unfolding electronic motion in such systems. We find that scattering patterns, obtained by X-ray time-resolved imaging from an electronic wavepacket, encode spatial and temporal correlations that deviate substantially from the common notion of the instantaneous electronic density as the key quantity being probed. Surprisingly, the patterns provide an unusually visual manifestation of the quantum nature of light. This quantum nature becomes central only for non-stationary electronic states and has profound consequences for time-resolved imaging.
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“It has been demonstrated that, even at low intensity, ultrafast x-ray scattering from electron wavepackets can hold surprises, which derive from the impossibility to separate electronically elastic and inelastic scattering events when using ultrafast x-ray pulses [116].”
From Roadmap of ultrafast x-ray atomic and molecular physics (2018) · cites this paper as [116]
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Research works printed but not linked: 1
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Dispersive Fourier transformation for fast continuous single-shot measurements
Goda, K., & Jalali, B. (2013) · Nature Photonics · doi:10.1038/nphoton.2012.359 · Cited by 1,013
Roadmap of ultrafast x-ray atomic and molecular physics
Young, L., Ueda, K., Gühr, M., Bucksbaum, P. H., Simon, M., Mukamel, S., Rohringer, N., Prince, K. C., Masciovecchio, C., Meyer, M., et al. (2018) · Journal of Physics B: Atomic, Molecular and Optical Physics · doi:10.1088/1361-6455/aa9735 · Cited by 337
Self-citationImaging Molecular Motion: Femtosecond X-Ray Scattering of an Electrocyclic Chemical Reaction
Minitti, M. P., Budarz, J. M., Kirrander, A., Robinson, J. S., Ratner, D., Lane, T. J., Zhu, D., Glownia, J. M., Kozina, M., Lemke, H. T., et al. (2015) · Physical Review Letters · doi:10.1103/physrevlett.114.255501 · Cited by 318
Ultrafast correlation-driven electron dynamics
Kuleff, A. I., & Cederbaum, L. S. (2014) · Journal of Physics B Atomic Molecular and Optical Physics · doi:10.1088/0953-4075/47/12/124002 · Cited by 173
Self-Referenced Coherent Diffraction X-Ray Movie of Ångstrom- and Femtosecond-Scale Atomic Motion
Glownia, J. M., Natan, A., Cryan, J. P., Hartsock, R., Kozina, M., Minitti, M. P., Nelson, S., Robinson, J., Sato, T., van Driel, T., et al. (2016) · Physical Review Letters · doi:10.1103/physrevlett.117.153003 · Cited by 149
Metadata
- Authors
- Dixit, G., Vendrell, O., & Santra, R.
- Affiliations
- Deutsches Elektronen-Synchrotron DESY (DE)
- Universität Hamburg (DE)
- Venue
- Proceedings of the National Academy of Sciences
- Publisher
- National Academy of Sciences
- Published
- 2012-07-02
- Volume
- 109
- Issue
- 29
- Pages
- 11636-11640
- ISSN
- 0027-8424 (ISSN-L)
- 1091-6490
- PMC
- PMC3406851
- OpenAlex
- W2533628335
- Cited by
- 177
- References
- 43
- Citations by year
- 2026: 7 · 2025: 8 · 2024: 18 · 2023: 19 · 2022: 14 · 2021: 14 · 2020: 13 · 2019: 11 · 2018: 13 · 2017: 11 · 2016: 6 · 2015: 8 · 2014: 19 · 2013: 12 · 2012: 4
- FWCI
- 7.11
- Type
- journal article
- Language
- en
- Open access
- green
- www.ncbi.nlm.nih.gov
- Locations
- Proceedings of the National Academy of Sciences (publishedVersion)
- Europe PMC (PubMed Central) (publishedVersion)
- PubMed Central (publishedVersion)
- PubMed (publishedVersion)
- Desy publication database (The Deutsches Elektronen-Synchrotron) (publishedVersion)
- arXiv (Cornell University) (submittedVersion)
- arXiv (Cornell University)
- Topics
- Physical Sciences › Physics and Astronomy › Atomic and Molecular Physics, and Optics › Laser-Matter Interactions and Applications
- Physical Sciences › Physics and Astronomy › Radiation › Advanced X-ray Imaging Techniques
- Physical Sciences › Physics and Astronomy › Radiation › X-ray Spectroscopy and Fluorescence Analysis
- Keywords
- time-resolved X-ray imaging, electron wave packets, spatio-temporal correlation, quantum nature of light, bond breaking and formation, charge migration
- MeSH terms
- Electrons, Light, Models, Chemical, Quantum Theory, Radiography, Scattering, Radiation
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