Cited by 132Atmospheric chemistry and aerosolsAtmospheric Ozone and ClimateAtmospheric and Environmental Gas Dynamics

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Climate-driven ground-level ozone extreme in the fall over the Southeast United States

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Zhang, Yuzhong, Wang, Yuhang·2016·Proceedings of the National Academy of Sciences

DOI 10.1073/pnas.1602563113PMC PMC5018760

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Abstract

Ground-level ozone is adverse to human and vegetation health. High ground-level ozone concentrations usually occur over the United States in the summer, often referred to as the ozone season. However, observed monthly mean ozone concentrations in the southeastern United States were higher in October than July in 2010. The October ozone average in 2010 reached that of July in the past three decades (1980-2010). Our analysis shows that this extreme October ozone in 2010 over the Southeast is due in part to a dry and warm weather condition, which enhances photochemical production, air stagnation, and fire emissions. Observational evidence and modeling analysis also indicate that another significant contributor is enhanced emissions of biogenic isoprene, a major ozone precursor, from water-stressed plants under a dry and warm condition. The latter finding is corroborated by recent laboratory and field studies. This climate-induced biogenic control also explains the puzzling fact that the two extremes of high October ozone both occurred in the 2000s when anthropogenic emissions were lower than the 1980s and 1990s, in contrast to the observed decreasing trend of July ozone in the region. The occurrences of a drying and warming fall, projected by climate models, will likely lead to more active photochemistry, enhanced biogenic isoprene and fire emissions, an extension of the ozone season from summer to fall, and an increase of secondary organic aerosols in the Southeast, posing challenges to regional air quality management.

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Authors: Zhang, Y., & Wang, Y.
Affiliations: Georgia Institute of Technology (US)
ORCID: Zhang, Yuzhong
Wang, Yuhang
Venue: Proceedings of the National Academy of Sciences
Publisher: National Academy of Sciences
Published: 2016-08-22
Volume: 113
Issue: 36
Pages: 10025-10030
ISSN: 0027-8424 (ISSN-L)
1091-6490
DOI: 10.1073/pnas.1602563113
PMC: PMC5018760
OpenAlex: W2515872853
Cited by: 132
References: 58
Citations by year: 2026: 5 · 2025: 6 · 2024: 11 · 2023: 17 · 2022: 19 · 2021: 27 · 2020: 10 · 2019: 13 · 2018: 10 · 2017: 14
FWCI: 7.51
Type: journal article
Language: en
Open access: green
www.ncbi.nlm.nih.gov
Licence: www.pnas.org/preview_site/misc/userlicense.xhtml (vor)
Locations: Proceedings of the National Academy of Sciences (publishedVersion)
PubMed Central (publishedVersion)
PubMed (publishedVersion)
Funders: Environmental Protection Agency (RD-83520401)
Topics: Physical Sciences › Earth and Planetary Sciences › Atmospheric Science › Atmospheric chemistry and aerosols
Physical Sciences › Earth and Planetary Sciences › Atmospheric Science › Atmospheric Ozone and Climate
Physical Sciences › Environmental Science › Global and Planetary Change › Atmospheric and Environmental Gas Dynamics
Keywords: surface ozone, climate change, isoprene emissions, photochemical ozone formation, fire emissions, air stagnation, secondary organic aerosol, air quality, southeastern United States, climate change projections
MeSH terms: Wildfires, Air Pollutants, Air Pollution, Butadienes, Environmental Monitoring, Humans, Ozone, Pentanes, Plants, Seasons, Weather, Southeastern United States, Models, Statistical, Hemiterpenes, Droughts

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Climate-driven ground-level ozone extreme in the fall over the Southeast United States

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