The DOI matches its Crossref record; 4 of the 4 references it cites were found in a registry or an index.
Spatially separating redox centers on 2D carbon nitride with cobalt single atom for photocatalytic H 2 O 2 production
Open accessAbstract
Significance: Photocatalysts frequently require simultaneous loading of oxidative and reductive cocatalysts to achieve both efficient half-reactions within a single material. Nevertheless, unregulated loading and distribution of two cocatalysts will result in direct contact between oxidation and reduction centers, leading to detrimental charge recombination. This research presents a center/edge approach to load two redox cocatalysts with controlled physical separation in atomistic scale using single-atom architecture. This spatial separation is critical for enhancing surface charge separation and achieving efficient H 2 O 2 production. We report that redox cocatalysts are spatially separated on a two-dimensional (2D) photocatalyst, which opens an approach for achieving both efficient oxidation and reduction reactions on 2D photocatalysts.
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Cites
Semiconductor-based Photocatalytic Hydrogen Generation
Chen, X., Shen, S., Guo, L., & Mao, S. S. (2010) · Chemical Reviews · doi:10.1021/cr1001645 · Cited by 7,876
Ong, W.-J., Tan, L.-L., Ng, Y. H., Yong, S.-T., & Chai, S.-P. (2016) · Chemical Reviews · doi:10.1021/acs.chemrev.6b00075 · Cited by 7,147
Metal-free efficient photocatalyst for stable visible water splitting via a two-electron pathway
Liu, J., Liu, Y., Liu, N., Han, Y., Zhang, X., Huang, H., Lifshitz, Y., Lee, S.-T., Zhong, J., & Kang, Z. (2015) · Science · doi:10.1126/science.aaa3145 · Cited by 4,468
A Particulate Photocatalyst Water-Splitting Panel for Large-Scale Solar Hydrogen Generation
Goto, Y., Hisatomi, T., Wang, Q., Higashi, T., Ishikiriyama, K., Maeda, T., Sakata, Y., Okunaka, S., Tokudome, H., Katayama, M., et al. (2018) · Joule · doi:10.1016/j.joule.2017.12.009 · Cited by 754
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Cited by
Chen, F., Liu, L.-L., Chen, J.-J., Li, W.-W., Chen, Y.-P., Zhang, Y.-J., Wu, J.-H., Mei, S.-C., Yang, Q., & Yu, H.-Q. (2021) · Water Research · doi:10.1016/j.watres.2020.116799 · Cited by 482
Photocatalytic H2O2 production Systems: Design strategies and environmental applications
Chen, Z., Yao, D., Chu, C., & Mao, S. (2023) · Chemical Engineering Journal · doi:10.1016/j.cej.2022.138489 · Cited by 482
Self-citationLi, S., Wang, C., Cai, M., Yang, F., Liu, Y., Chen, J., Zhang, P., Li, X., & Chen, X. (2022) · Chemical Engineering Journal · doi:10.1016/j.cej.2021.131158 · Cited by 470
Enhanced Photocatalytic H2O2 Production over Carbon Nitride by Doping and Defect Engineering
Wu, S., Yu, H., Chen, S., & Quan, X. (2020) · ACS Catalysis · doi:10.1021/acscatal.0c03359 · Cited by 466
Qi, Y., Zhang, J., Kong, Y., Zhao, Y., Chen, S., Li, D., Liu, W., Chen, Y., Xie, T., Cui, J., et al. (2022) · Nature Communications · doi:10.1038/s41467-022-28146-6 · Cited by 429
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Metadata
- Authors
- Chu, C., Zhu, Q., Pan, Z., Gupta, S., Huang, D., Du, Y., Weon, S., Wu, Y., Muhich, C., Stavitski, E., Domen, K., & Kim, J.-H.
- Venue
- Proceedings of the National Academy of Sciences
- Published
- 2020-03-11
- Volume
- 117
- Issue
- 12
- Pages
- 6376-6382
- ISSN
- 0027-8424 (ISSN-L)
- 1091-6490
- OpenAlex
- W3011260827
- Cited by
- 400
- References
- 4
- FWCI
- 10.99
- Type
- journal article
- Language
- en
- Open access
- hybrid
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- Chu, C., Zhu, Q., Pan, Z., Gupta, S., Huang, D., Du, Y., Weon, S., Wu, Y., Muhich, C., Stavitski, E., Domen, K., & Kim, J.-H. (2020). Spatially separating redox centers on 2D carbon nitride with cobalt single atom for photocatalytic H 2 O 2 production. Proceedings of the National Academy of Sciences. https://doi.org/10.1073/pnas.1913403117
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