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Advanced Oxidation Processes for Wastewater Treatment: Formation of Hydroxyl Radical and Application
Abstract
Advanced oxidation processes (AOPs), defined as those technologies that utilize the hydroxyl radical (·OH) for oxidation, have received increasing attention in the research and development of wastewater treatment technologies in the last decades. These processes have been applied successfully for the removal or degradation of toxic pollutants or used as pretreatment to convert recalcitrant pollutants into biodegradable compounds that can then be treated by conventional biological methods. The efficacy of AOPs depends on the generation of reactive free radicals, the most important of which is the hydroxyl radical (·OH). The authors summarize the formation reactions of ·OH and the mechanisms of pollutants degradation. They cover six types of advanced oxidation processes, including radiation, photolysis and photocatalysis, sonolysis, electrochemical oxidation technologies, Fenton-based reactions, and ozone-based processes. Controversial issues in pollutants degradation mechanism were discussed. They review the application of these processes for removal of different kinds of toxic pollutants from wastewater, including aromatic compounds, dyes, pharmaceutical compounds, and pesticides, with emphasis on the parameters assessed, removal effectiveness, and the degradation mechanisms of pollutants. The authors discuss issues associated with practical wastewater treatment and offer suggestions for the direction for future researches.
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“The degradation of contaminants and their derivatives by various AOPs, such as UV/H2O2 photolysis, photocatalysis, Fenton, electro-Fenton or cavitation-based methods, etc., resulted in good degradation and mineralization efficiency [11-16].”
From Advanced Oxidation Processes for Degradation of Water Pollutants—Ambivalent Impact of Carbonate Species: A Review (2023) · cites this paper as [12]
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Self-citationLee, C., Remucal, C. K., & Sedlak, D. L. (2008) · Environmental Science & Technology · doi:10.1021/es802169g · Cited by 2
Flagged first, then by citations
Research works printed but not linked: 3
- Ensminger D., 1973, Ultrasonic: The low and high-intensity-applications
- Nemes A., 2000, Inorg. React. Mech.,, 2, 327
- 10.1016/S1010-6030(01)00368-9 · DOI
Cited by
Sorted by citations
Wang, J., & Wang, S. (2018) · Chemical Engineering Journal · doi:10.1016/j.cej.2017.11.059 · Cited by 4,087
Self-citationGhanbari, F., & Moradi, M. (2016) · Chemical Engineering Journal · doi:10.1016/j.cej.2016.10.064 · Cited by 2,670
Advanced Oxidation Processes in Water/Wastewater Treatment: Principles and Applications. A Review
Oturan, M. A., & Aaron, J. (2014) · Critical Reviews in Environmental Science and Technology · doi:10.1080/10643389.2013.829765 · Cited by 2,304
Environmental Implications of Hydroxyl Radicals ( • OH)
Gligorovski, S., Strekowski, R., Barbati, S., & Vione, D. V. (2015) · Chemical Reviews · doi:10.1021/cr500310b · Cited by 1,672
Reactive Species in Advanced Oxidation Processes: Formation, Identification and Reaction Mechanism
Wang, J., & Wang, S. (2020) · Chemical Engineering Journal · doi:10.1016/j.cej.2020.126158 · Cited by 1,585
Self-citation
Metadata
- Authors
- WANG, J. L., & XU, L. J.
- Affiliations
- Tsinghua University (CN)
- Venue
- Critical Reviews in Environmental Science and Technology
- Publisher
- Informa UK Limited
- Published
- 2012-02
- Volume
- 42
- Issue
- 3
- Pages
- 251-325
- ISSN
- 1064-3389 (ISSN-L)
- 1547-6537
- OpenAlex
- W2040456488
- Cited by
- 1,586
- References
- 317
- Citations by year
- 2026: 88 · 2025: 124 · 2024: 154 · 2023: 174 · 2022: 188 · 2021: 194 · 2020: 160 · 2019: 143 · 2018: 100 · 2017: 83 · 2016: 57 · 2015: 44 · 2014: 42 · 2013: 28 · 2012: 7
- FWCI
- 23.95
- Type
- journal article
- Language
- en
- Open access
- closed
- Locations
- Critical Reviews in Environmental Science and Technology (publishedVersion)
- Topics
- Physical Sciences › Environmental Science › Water Science and Technology › Advanced oxidation water treatment
- Physical Sciences › Environmental Science › Environmental Engineering › Environmental remediation with nanomaterials
- Physical Sciences › Chemical Engineering › Process Chemistry and Technology › Subcritical and Supercritical Water Processes
- Keywords
- advanced oxidation processes, hydroxyl radicals, wastewater treatment, pollutant degradation mechanisms, photocatalysis, sonolysis, electrochemical oxidation, Fenton reaction, ozonation, radiation-induced oxidation, dye degradation, pharmaceutical pollutants, pesticide removal, aromatic compounds, recalcitrant pollutants, biodegradability
About these checks
Registry, retraction, Cites and statistics results are computed, not judged, with one exception: a printed reference that no index lists is read once by a model before it counts as a citation error. Claims are extracted by a model and kept only when their quote appears verbatim in the text; each cited source is then checked, with a model’s help, for whether it says what the claim relies on. Those verdicts can be wrong — read the claim’s quote and the cited source before relying on one.
Statistics and arithmetic are recomputed, not judged.
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