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ACTINIDE PARTITIONING—A REVIEW
Abstract
Reagents and methods that have been developed during the past 20 years for hydrometallurgical partitioning of actinides from different types of transuranium (TRU) wastes and dissolved fuels are reviewed. Emphasis is placed on the extraction performance of the fully-optimized reagents rather than on the structural iterations that were undertaken (and in some cases are still being conducted) to identify the optimum species. Particular attention is paid to separation processes that have been demonstrated in batch and counter-current solvent extraction, and batch and column mode extraction chromatography. The salient features of the various techniques and reagents for actinide recycle are compared. Sections of the review focus on neptunium behavior in hydrometallurgy and on characterization of those reagents best suited to the separation of trivalent actinides from fission product lanthanides. Selected flowsheets that have been reported for the separation and recovery of actinides from TRU wastes are presented.
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Cited by
Ligands for f-element extraction used in the nuclear fuel cycle
Leoncini, A., Huskens, J., & Verboom, W. (2017) · Chemical Society Reviews · doi:10.1039/c7cs00574a · Cited by 486
Ansari, S. A., Pathak, P. N., Manchanda, V. K., Husain, M., Prasad, A. K., & Parmar, V. S. (2005) · Solvent Extraction and Ion Exchange · doi:10.1081/sei-200066296 · Cited by 420
Paiva, A. P., & Malik, P. (2004) · Journal of Radioanalytical and Nuclear Chemistry · doi:10.1023/b:jrnc.0000034890.23325.b5 · Cited by 290
Exploiting outer-sphere interactions to enhance metal recovery by solvent extraction
Turkington, J. R., Bailey, P. J., Love, J. B., Wilson, A. M., & Tasker, P. A. (2013) · Chemical Communications · doi:10.1039/c2cc37874d · Cited by 63
Mesoscopic Aspects of Phase Transitions in a Solvent Extraction System
Ellis, R. J., Audras, M., & Antonio, M. R. (2012) · Langmuir · doi:10.1021/la3034879 · Cited by 42
Metadata
- Authors
- Mathur, J. N., Murali, M. S., & Nash, K. L.
- Venue
- Solvent Extraction and Ion Exchange
- Publisher
- Informa UK Limited
- Published
- 2001-05-31
- Volume
- 19
- Issue
- 3
- Pages
- 357-390
- ISSN
- 0736-6299 (ISSN-L)
- 1532-2262
- OpenAlex
- W2008150552
- Cited by
- 528
- References
- 0
- FWCI
- 5.63
- Type
- journal article
- Language
- en
- Open access
- closed
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- Mathur, J. N., Murali, M. S., & Nash, K. L. (2001). ACTINIDE PARTITIONING—A REVIEW. Solvent Extraction and Ion Exchange. https://doi.org/10.1081/sei-100103276
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