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Self-probing of molecules with high harmonic generation
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This tutorial presents the most important aspects of the molecular self-probing paradigm, which views the process of high harmonic generation as "a molecule being probed by one of its own electrons". Since the properties of the electron wavepacket acting as a probe allow a combination of attosecond and Ångström resolutions in measurements, this idea bears great potential for the observation, and possibly control, of ultrafast quantum dynamics in molecules at the electronic level. Theoretical as well as experimental methods and concepts at the basis of self-probing measurements are introduced. Many of these are discussed on the example of molecular orbital tomography.
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Metadata
- Authors
- Haessler, S., Caillat, J., & Salières, P.
- Affiliations
- TU Wien (AT)
- Centre National de la Recherche Scientifique (FR)
- Venue
- Journal of Physics B: Atomic, Molecular and Optical Physics
- Publisher
- IOP Publishing
- Published
- 2011-09-26
- Volume
- 44
- Issue
- 20
- Pages
- 203001
- ISSN
- 0953-4075 (ISSN-L)
- 1361-6455
- OpenAlex
- W1972030855
- Cited by
- 149
- References
- 231
- Citations by year
- 2025: 1 · 2024: 4 · 2023: 4 · 2022: 3 · 2021: 7 · 2020: 7 · 2019: 6 · 2018: 19 · 2017: 8 · 2016: 19 · 2015: 12 · 2014: 18 · 2013: 21 · 2012: 17
- FWCI
- 10.24
- Type
- journal article
- Language
- en
- Open access
- green
- arxiv.org
- Locations
- Journal of Physics B Atomic Molecular and Optical Physics (publishedVersion)
- arXiv (Cornell University) (submittedVersion)
- HAL (submittedVersion, other-oa)
- arXiv (Cornell University)
- Funders
- Agence Nationale de la Recherche (ANR-09-BLAN-0031)
- Topics
- Physical Sciences › Physics and Astronomy › Atomic and Molecular Physics, and Optics › Laser-Matter Interactions and Applications
- Physical Sciences › Physics and Astronomy › Atomic and Molecular Physics, and Optics › Spectroscopy and Quantum Chemical Studies
- Physical Sciences › Engineering › Electrical and Electronic Engineering › Terahertz technology and applications
- Keywords
- high harmonic generation, molecular dynamics, strong-field ionization, attosecond pulses
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