Controlling core hole relaxation dynamics via intense optical fields
Open accessAbstract
The influence of an intense optical laser on the electronic relaxation of the 3d–5p resonance in atomic Kr has been studied experimentally and theoretically. The resonance profile undergoes a strong modification, observed as a shift and a broadening of the excitation spectrum, as a function of the optical intensity. The theoretical treatment of the process demonstrates the importance of strongly time-dependent dynamics as the origin of the observed phenomena resulting in the ponderomotive shift of the resonance position as well as a competition between resonant and normal Auger decay. The ionization of the excited 5p electron by the optical laser provides the possibility to change the ratio between singly and doubly charged final states by controlling the relaxation of the resonant core hole state via resonant or normal Auger decay.
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Changes in the dynamics of autoionizing resonances can be induced by the presence of a strong XUV or external optical field.
“Changes in the dynamics of autoionizing resonances induced by the presence of a strong XUV or external optical field [78] highlighted the possibilities”
From Roadmap of ultrafast x-ray atomic and molecular physics (2018) · cites this paper as [78]
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Roadmap of ultrafast x-ray atomic and molecular physics
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- Authors
- Mazza, T., Papamihail, K. G., Radcliffe, P., Li, W. B., Kelly, T. J., Costello, J. T., Düsterer, S., Lambropoulos, P., & Meyer, M.
- Affiliations
- European X-Ray Free-Electron Laser (DE)
- University of Crete (GR)
- Tongji University (CN)
- Dublin City University (IE)
- Deutsches Elektronen-Synchrotron DESY (DE)
- Corresponding author
- Meyer, M
- Venue
- Journal of Physics B: Atomic, Molecular and Optical Physics
- Publisher
- IOP Publishing
- Published
- 2012-07-02
- Volume
- 45
- Issue
- 14
- Pages
- 141001
- ISSN
- 0953-4075 (ISSN-L)
- 1361-6455
- OpenAlex
- W2009082314
- Cited by
- 18
- References
- 25
- Citations by year
- 2022: 1 · 2019: 2 · 2018: 1 · 2017: 2 · 2016: 1 · 2015: 3 · 2014: 1 · 2013: 4 · 2012: 3
- FWCI
- 1.82
- Type
- journal article
- Language
- en
- Open access
- bronze
- doi.org
- Locations
- Journal of Physics B Atomic Molecular and Optical Physics (publishedVersion)
- Desy publication database (The Deutsches Elektronen-Synchrotron) (publishedVersion)
- European XFEL (submittedVersion)
- Funders
- Science Foundation Ireland (PI 07/IN.1/I1771, 07/IN.1/I1771)
- National Natural Science Foundation of China
- Topics
- Physical Sciences › Physics and Astronomy › Atomic and Molecular Physics, and Optics › Laser-Matter Interactions and Applications
- Physical Sciences › Physics and Astronomy › Atomic and Molecular Physics, and Optics › Atomic and Molecular Physics
- Physical Sciences › Physics and Astronomy › Radiation › X-ray Spectroscopy and Fluorescence Analysis
- Keywords
- core-hole relaxation, Auger decay, resonant Auger decay, time-dependent dynamics, multiphoton ionization
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