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Nuclear Motions Associated with Electron Transitions in Diatomic Molecules
Abstract
The question of nuclear motions associated with electron transitions is discussed from the standpoint of quantum mechanics. It appears that Heisenberg's indetermination principle gives the clue to the inexactness of the earlier method based on Franck's postulate since its strict application calls for a violation of the principle. The existence of an entirely new type of band spectrum due to the wave nature of matter is predicted and the interpretation of Rayleigh's mercury band at 2476-2482 A.U. as of this type is suggested. Finally it is shown that while Franck's postulate is also true for electron jumps in atoms, it is of but trivial interest because its inexactness is much greater for the electrons than for heavy nuclei.
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Citations
Cites
�ber den anschaulichen Inhalt der quantentheoretischen Kinematik und Mechanik
Heisenberg, W. (1927) · Zeitschrift f�r Physik · doi:10.1007/bf01397280 · Cited by 4,278
The Quantum Postulate and the Recent Development of Atomic Theory1
BOHR, N. (1928) · Nature · doi:10.1038/121580a0 · Cited by 1,700
Cited by
Colloquium: Coherently controlled adiabatic passage
Král, P., Thanopulos, I., & Shapiro, M. (2007) · Reviews of Modern Physics · doi:10.1103/revmodphys.79.53 · Cited by 444
Baiardi, A., Bloino, J., & Barone, V. (2013) · Journal of Chemical Theory and Computation · doi:10.1021/ct400450k · Cited by 423
Quantum mechanical tunnelling in biological systems
Devault, D. (1980) · Quarterly Reviews of Biophysics · doi:10.1017/s003358350000175x · Cited by 406
Dynamical symmetry of vibronic transitions in polyatomic molecules and the Franck-Condon principle
Doktorov, E. V., Malkin, I. A., & Man'ko, V. I. (1977) · Journal of Molecular Spectroscopy · doi:10.1016/0022-2852(77)90269-7 · Cited by 359
Neese, F., Petrenko, T., Ganyushin, D., & Olbrich, G. (2007) · Coordination Chemistry Reviews · doi:10.1016/j.ccr.2006.05.019 · Cited by 332
Metadata
- Authors
- Condon, E. U.
- Venue
- Physical Review
- Publisher
- American Physical Society (APS)
- Published
- 1928-12-01
- Volume
- 32
- Issue
- 6
- Pages
- 858-872
- ISSN
- 0031-899X (ISSN-L)
- OpenAlex
- W2066148764
- Cited by
- 841
- References
- 2
- FWCI
- 6.22
- Type
- journal article
- Language
- en
- Open access
- closed
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