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K-shell photoabsorption of theN2molecule
Abstract
The K-shell photoabsorption spectrum of the ${\mathrm{N}}_{2}$ molecule, recorded with unprecedented energy resolution and statistical accuracy, reveals several new Rydberg transitions and double-excitation states. The nearly identical term values, vibrational frequencies and internuclear separations of the 1s-excited states of ${\mathrm{N}}_{2}$ and of the 2\ensuremath{\pi}-excited states of NO, allow for a complete peak assignment for the ${\mathrm{N}}_{2}$ Rydberg series and strongly support both the core-hole localization picture and equivalent-core model. Subtle differences are related to the final-state charge distribution in the vicinity of the nuclei and to the bonding character of the valence orbitals.
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Citations
Cited by
Charge-transfer dynamics studied using resonant core spectroscopies
Brühwiler, P. A., Karis, O., & Mårtensson, N. (2002) · Reviews of Modern Physics · doi:10.1103/revmodphys.74.703 · Cited by 372
Metadata
- Authors
- Chen, C. T., Ma, Y., & Sette, F.
- Venue
- Physical Review A
- Publisher
- American Physical Society (APS)
- Published
- 1989-12-01
- Volume
- 40
- Issue
- 11
- Pages
- 6737-6740
- ISSN
- 0556-2791 (ISSN-L)
- OpenAlex
- W2065861873
- Cited by
- 276
- References
- 0
- FWCI
- 16.54
- Type
- journal article
- Language
- en
- Open access
- closed
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- Chen, C. T., Ma, Y., & Sette, F. (1989). K-shell photoabsorption of theN2molecule. Physical Review A. https://doi.org/10.1103/physreva.40.6737
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
Semantic Scholar’s data is described in: Kinney, R., et al. (2023). The Semantic Scholar Open Data Platform. arXiv:2301.10140.
