The DOI matches its Crossref record; 77 of the 77 references it cites were found in a registry or an index.
Quantitative rescattering theory for high-order harmonic generation from molecules
Open accessAbstract
The quantitative rescattering theory (QRS) for high-order harmonic generation (HHG) by intense laser pulses is presented. According to the QRS, HHG spectra can be expressed as a product of a returning electron wave packet and the photorecombination differential cross section of the laser-free continuum electron back to the initial bound state. We show that the shape of the returning electron wave packet is determined mostly by the laser. The returning electron wave packets can be obtained from the strong-field approximation or from the solution of the time-dependent Schr\"odinger equation (TDSE) for a reference atom. The validity of the QRS is carefully examined by checking against accurate results for both harmonic magnitude and phase from the solution of the TDSE for atomic targets within the single active electron approximation. Combining with accurate transition dipoles obtained from state-of-the-art molecular photoionization calculations, we further show that available experimental measurements for HHG from partially aligned molecules can be explained by the QRS. Our results show that quantitative description of the HHG from aligned molecules has become possible. Since infrared lasers of pulse durations of a few femtoseconds are easily available in the laboratory, they may be used for dynamic imaging of a transient molecule with femtosecond temporal resolutions.
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Cites
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Kraus, P. M., Mignolet, B., Baykusheva, D., Rupenyan, A., Horný, L., Penka, E. F., Grassi, G., Tolstikhin, O. I., Schneider, J., Jensen, F., et al. (2015) · Science · doi:10.1126/science.aab2160 · Cited by 628
Attosecond molecular dynamics: fact or fiction?
Lépine, F., Ivanov, M. Y., & Vrakking, M. J. J. (2014) · Nature Photonics · doi:10.1038/nphoton.2014.25 · Cited by 428
Strong-field rescattering physics—self-imaging of a molecule by its own electrons
Lin, C. D., Le, A.-T., Chen, Z., Morishita, T., & Lucchese, R. (2010) · Journal of Physics B: Atomic, Molecular and Optical Physics · doi:10.1088/0953-4075/43/12/122001 · Cited by 288
Self-citationSpatiotemporal isolation of attosecond soft X-ray pulses in the water window
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Metadata
- Authors
- Le, A.-T., Lucchese, R. R., Tonzani, S., Morishita, T., & Lin, C. D.
- Venue
- Physical Review A
- Publisher
- American Physical Society (APS)
- Published
- 2009-07-01
- Volume
- 80
- Issue
- 1
- ISSN
- 0556-2791 (ISSN-L)
- 1050-2947
- 1094-1622
- OpenAlex
- W2045565918
- Cited by
- 366
- References
- 77
- FWCI
- 16.36
- Type
- journal article
- Language
- en
- Open access
- bronze
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