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Temperature- and pressure-induced spin-state transitions inLaCoO3
Open accessAbstract
We report the continuous variation of the spin moment of cobalt in ${\mathrm{LaCoO}}_{3}$ across its temperature and pressure-induced spin transitions evidenced with $K\ensuremath{\beta}$ emission spectra. The first thermal transition is best described by a transition to an orbitally nondegenerate intermediate spin $(S=1)$ state. In parallel, continuous redistribution of the $3d$ electrons is also indicated by partial fluorescence yield x-ray absorption spectra. At high pressure, our study confirms that the material becomes low spin between 40 and 70 kbar at room temperature.
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Cited by
Vankó, G., Neisius, T., Molnár, G., Renz, F., Kárpáti, S., Shukla, A., & de Groot, F. M. F. (2006) · The Journal of Physical Chemistry B · doi:10.1021/jp0615961 · Cited by 320
Self-citationSpin states of metal centers in electrocatalysis
Zhang, Y., Wu, Q., Seow, J. Z. Y., Jia, Y., Ren, X., & Xu, Z. J. (2024) · Chemical Society Reviews · doi:10.1039/d3cs00913k · Cited by 267
Kantor, I. Y., Dubrovinsky, L. S., & McCammon, C. A. (2006) · Physical Review B · doi:10.1103/physrevb.73.100101 · Cited by 72
Metadata
- Authors
- Vankó, G., Rueff, J.-P., Mattila, A., Németh, Z., & Shukla, A.
- Venue
- Physical Review B
- Publisher
- American Physical Society (APS)
- Published
- 2006-01-26
- Volume
- 73
- Issue
- 2
- ISSN
- 1098-0121 (ISSN-L)
- 1550-235X
- OpenAlex
- W1761883047
- Cited by
- 196
- References
- 0
- FWCI
- 7.55
- Type
- journal article
- Language
- en
- Open access
- green
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- Vankó, G., Rueff, J.-P., Mattila, A., Németh, Z., & Shukla, A. (2006). Temperature- and pressure-induced spin-state transitions inLaCoO3. Physical Review B. https://doi.org/10.1103/physrevb.73.024424
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