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Theory of neutral and charged excitons in monolayer transition metal dichalcogenides
Open accessAbstract
We present a microscopic theory of neutral excitons and charged excitons (trions) in monolayers of transition metal dichalcogenides, including molybdenum disulfide. Our theory is based on an effective mass model of excitons and trions, parameterized by ab initio calculations and incorporating a proper treatment of screening in two dimensions. The calculated exciton binding energies are in good agreement with high-level many-body computations based on the Bethe-Salpeter equation. Furthermore, our calculations for the more complex trion species compare very favorably with recent experimental measurements and provide atomistic insight into the microscopic features which determine the trion binding energy.
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Generalized Gradient Approximation Made Simple
Perdew, J. P., Burke, K., & Ernzerhof, M. (1996) · Physical Review Letters · doi:10.1103/physrevlett.77.3865 · Cited by 215,824
Two-dimensional atomic crystals
Novoselov, K. S., Jiang, D., Schedin, F., Booth, T. J., Khotkevich, V. V., Morozov, S. V., & Geim, A. K. (2005) · Proceedings of the National Academy of Sciences · doi:10.1073/pnas.0502848102 · Cited by 11,788
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Photonics and optoelectronics of 2D semiconductor transition metal dichalcogenides
Mak, K. F., & Shan, J. (2016) · Nature Photonics · doi:10.1038/nphoton.2015.282 · Cited by 3,819
Emerging Device Applications for Semiconducting Two-Dimensional Transition Metal Dichalcogenides
Jariwala, D., Sangwan, V. K., Lauhon, L. J., Marks, T. J., & Hersam, M. C. (2014) · ACS Nano · doi:10.1021/nn500064s · Cited by 2,753
Schaibley, J. R., Yu, H., Clark, G., Rivera, P., Ross, J. S., Seyler, K. L., Yao, W., & Xu, X. (2016) · Nature Reviews Materials · doi:10.1038/natrevmats.2016.55 · Cited by 2,652
Polaritons in layered two-dimensional materials
Low, T., Chaves, A., Caldwell, J. D., Kumar, A., Fang, N. X., Avouris, P., Heinz, T. F., Guinea, F., Martin-Moreno, L., & Koppens, F. (2017) · Nature Materials · doi:10.1038/nmat4792 · Cited by 1,317
Photovoltaic Effect in an Electrically Tunable van der Waals Heterojunction
Furchi, M. M., Pospischil, A., Libisch, F., Burgdörfer, J., & Mueller, T. (2014) · Nano Letters · doi:10.1021/nl501962c · Cited by 1,085
Metadata
- Authors
- Berkelbach, T. C., Hybertsen, M. S., & Reichman, D. R.
- Venue
- Physical Review B
- Publisher
- American Physical Society (APS)
- Published
- 2013-07-25
- Volume
- 88
- Issue
- 4
- ISSN
- 1098-0121 (ISSN-L)
- 1550-235X
- OpenAlex
- W2054773072
- Cited by
- 955
- References
- 2
- FWCI
- 25.01
- Type
- journal article
- Language
- en
- Open access
- green
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- Berkelbach, T. C., Hybertsen, M. S., & Reichman, D. R. (2013). Theory of neutral and charged excitons in monolayer transition metal dichalcogenides. Physical Review B. https://doi.org/10.1103/physrevb.88.045318
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