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α−RuCl3: A spin-orbit assisted Mott insulator on a honeycomb lattice
Open accessAbstract
We examine the role of spin-orbit coupling in the electronic structure of $\ensuremath{\alpha}\ensuremath{-}{\mathrm{RuCl}}_{3}$, in which Ru ions in $4{d}^{5}$ configuration form a honeycomb lattice. Our x-ray absorption spectroscopy measurements at the Ru $L$ edges exhibit distinct spectral features associated with the presence of substantial spin-orbit coupling, as well as an anomalously large branching ratio. Furthermore the measured optical spectra can be described very well with first-principles electronic structure calculations obtained by taking into account both spin-orbit coupling and electron correlations. We propose that $\ensuremath{\alpha}\ensuremath{-}{\mathrm{RuCl}}_{3}$ is a spin-orbit assisted Mott insulator, and that the bond-dependent Kitaev interaction may be important for understanding magnetism of this compound.
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Self-interaction correction to density-functional approximations for many-electron systems
Perdew, J. P., & Zunger, A. (1981) · Physical Review B · doi:10.1103/physrevb.23.5048 · Cited by 20,887
Anyons in an exactly solved model and beyond
Kitaev, A. (2006) · Annals of Physics · doi:10.1016/j.aop.2005.10.005 · Cited by 5,245
Wan, X., Turner, A. M., Vishwanath, A., & Savrasov, S. Y. (2011) · Physical Review B · doi:10.1103/physrevb.83.205101 · Cited by 4,718
Cited by
Proximate Kitaev quantum spin liquid behaviour in a honeycomb magnet
Banerjee, A., Bridges, C. A., Yan, J.-Q., Aczel, A. A., Li, L., Stone, M. B., Granroth, G. E., Lumsden, M. D., Yiu, Y., Knolle, J., et al. (2016) · Nature Materials · doi:10.1038/nmat4604 · Cited by 835
Recent progress on 2D magnets: Fundamental mechanism, structural design and modification
Jiang, X., Liu, Q., Xing, J., Liu, N., Guo, Y., Liu, Z., & Zhao, J. (2021) · Applied Physics Reviews · doi:10.1063/5.0039979 · Cited by 445
Successive magnetic phase transitions inα−RuCl3: XY-like frustrated magnet on the honeycomb lattice
Kubota, Y., Tanaka, H., Ono, T., Narumi, Y., & Kindo, K. (2015) · Physical Review B · doi:10.1103/physrevb.91.094422 · Cited by 317
Excitations in the field-induced quantum spin liquid state of α-RuCl3
Banerjee, A., Lampen-Kelley, P., Knolle, J., Balz, C., Aczel, A. A., Winn, B., Liu, Y., Pajerowski, D. M., Yan, J.-Q., Bridges, C. A., et al. (2017) · Apollo (University of Cambridge) · doi:10.17863/cam.11029 · Cited by 303
Neutron tomography of magnetic Majorana fermions in a proximate quantum spin liquid
Banerjee, A., Yan, J., Knolle, J., Bridges, C. A., Stone, M. B., Lumsden, M. D., Mandrus, D. G., Tennant, D. M., Moessner, R., & Nagler, S. E. (2016) · arXiv (Cornell University) · doi:10.48550/arxiv.1609.00103 · Cited by 258
Metadata
- Authors
- Plumb, K. W., Clancy, J. P., Sandilands, L. J., Shankar, V. V., Hu, Y. F., Burch, K. S., Kee, H.-Y., & Kim, Y.-J.
- Venue
- Physical Review B
- Publisher
- American Physical Society (APS)
- Published
- 2014-07-29
- Volume
- 90
- Issue
- 4
- ISSN
- 1098-0121 (ISSN-L)
- 1550-235X
- OpenAlex
- W2009820981
- Cited by
- 804
- References
- 3
- FWCI
- 24.89
- Type
- journal article
- Language
- en
- Open access
- green
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- Plumb, K. W., Clancy, J. P., Sandilands, L. J., Shankar, V. V., Hu, Y. F., Burch, K. S., Kee, H.-Y., & Kim, Y.-J. (2014). α−RuCl3: A spin-orbit assisted Mott insulator on a honeycomb lattice. Physical Review B. https://doi.org/10.1103/physrevb.90.041112
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