Cited by 1752D Materials and ApplicationsTopological Materials and PhenomenaAdvanced Condensed Matter Physics

Origin of the turn-on temperature behavior inWTe2

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Wang, Y. L., Thoutam, L. R., Xiao, Z. L., Hu, J., Das, S., Mao, Z. Q., Wei, J., Divan, R. +3 more·2015·Physical Review B

Abstract

A hallmark of materials with extremely large magnetoresistance (XMR) is the transformative turn-on temperature behavior: when the applied magnetic field $H$ is above certain value, the resistivity versus temperature $\ensuremath{\rho}(T)$ curve shows a minimum at a field dependent temperature ${T}^{*}$, which has been interpreted as a magnetic-field-driven metal-insulator transition or attributed to an electronic structure change. Here, we demonstrate that $\ensuremath{\rho}(T)$ curves with turn-on behavior in the newly discovered XMR material ${\mathrm{WTe}}_{2}$ can be scaled as $\text{MR}\ensuremath{\sim}{(H/{\ensuremath{\rho}}_{0})}^{m}$ with $m\ensuremath{\approx}2$ and ${\ensuremath{\rho}}_{0}$ being the resistivity at zero field. We obtained experimentally and also derived from the observed scaling the magnetic field dependence of the turn-on temperature ${T}^{*}\ensuremath{\sim}{(H\ensuremath{-}{H}_{c})}^{\ensuremath{\nu}}$ with $\ensuremath{\nu}\ensuremath{\approx}1/2$, which was earlier used as evidence for a predicted metal-insulator transition. The scaling also leads to a simple quantitative expression for the resistivity ${\ensuremath{\rho}}^{*}\ensuremath{\approx}2{\ensuremath{\rho}}_{0}$ at the onset of the XMR behavior, which fits the data remarkably well. These results exclude the possible existence of a magnetic-field-driven metal-insulator transition or significant contribution of an electronic structure change to the low-temperature XMR in ${\mathrm{WTe}}_{2}$. This work resolves the origin of the turn-on behavior observed in several XMR materials and also provides a general route for a quantitative understanding of the temperature dependence of MR in both XMR and non-XMR materials.

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Crossref · 10.1103/physrevb.92.180402

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  • Multiple oscillation frequencies are often observed in most topological semimetals, such as the TaAs family and WHM materials with PbFCl-type structure.

    “However, multiple oscillation frequencies are often observed in most topological semimetals, such as those of the TaAs family (179, 180, 182, 183, 191-193, 227, 243) and WHM materials with PbFCl-type structure (W = Zr or Hf; H = Si, Ge, or Sn; M = S, Se, or Te) (156,221,222,226,228,232,233,241,242,244,245).”

    From Transport of Topological Semimetals (2019) · cites this paper as [182]

    The discussion on p. 4 mentions quantum-oscillation measurements only to compare electron and hole carrier densities in WTe₂. The introduction (p. 1) mentions TaAs but does not discuss its oscillation frequencies. Searches for multiple frequencies and PbFCl-type WHM materials found no passage addressing the attributed claim. (LLM, conf=0.76)

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Research works printed but not linked: 9

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Authors
Wang, Y. L., Thoutam, L. R., Xiao, Z. L., Hu, J., Das, S., Mao, Z. Q., Wei, J., Divan, R., Luican-Mayer, A., Crabtree, G. W., & Kwok, W. K.
Affiliations
  • University of Notre Dame (US)
  • Northern Illinois University (US)
  • Tulane University (US)
  • Argonne National Laboratory (US)
Venue
Physical Review B
Published
2015-11-03
Volume
92
Issue
18
ISSN
  • 1098-0121 (ISSN-L)
  • 1550-235X
OpenAlex
W2139562289
Cited by
175
References
1
Citations by year
2026: 7 · 2025: 16 · 2024: 17 · 2023: 13 · 2022: 17 · 2021: 19 · 2020: 20 · 2019: 14 · 2018: 20 · 2017: 20 · 2016: 12
FWCI
7.04
Type
journal article
Language
en
Open access
Locations
  • Physical Review B (publishedVersion)
  • arXiv (Cornell University) (submittedVersion)
  • Figshare (submittedVersion)
  • OSTI OAI (U.S. Department of Energy Office of Scientific and Technical Information) (submittedVersion)
  • arXiv (Cornell University)
Funders
  • U.S. Department of Energy (DE-AC02-06CH11357)
  • National Science Foundation (DMR-1407175, DMR-1205469)
  • Tulane University
  • Louisiana Board of Regents (LEQSF(2014-15)-ENH-TR-24)
Topics
  • Physical Sciences › Materials Science › Materials Chemistry › 2D Materials and Applications
  • Physical Sciences › Physics and Astronomy › Atomic and Molecular Physics, and Optics › Topological Materials and Phenomena
  • Physical Sciences › Physics and Astronomy › Condensed Matter Physics › Advanced Condensed Matter Physics
Keywords
WTe2, resistivity scaling, metal-insulator transition, temperature dependence of magnetoresistance, two-dimensional transition metal dichalcogenides, electronic structure

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