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Equilibrium free-energy differences from nonequilibrium measurements: A master-equation approach
Open accessAbstract
In has recently been shown that the Helmholtz free-energy difference between two equilibrium configurations of a system may be obtained from an ensemble of finite-time (nonequilibrium) measurements of the work performed in switching an external parameter of the system. Here this result is established, as an identity, within the master equation formalism. Examples are discussed and numerical illustrations provided.
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Cites
Equation of State Calculations by Fast Computing Machines
Metropolis, N., Rosenbluth, A. W., Rosenbluth, M. N., Teller, A. H., & Teller, E. (1953) · The Journal of Chemical Physics · doi:10.1063/1.1699114 · Cited by 37,192
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Metadata
- Authors
- Jarzynski, C.
- Venue
- Physical Review E
- Publisher
- American Physical Society (APS)
- Published
- 1997-11-01
- Volume
- 56
- Issue
- 5
- Pages
- 5018-5035
- ISSN
- 1063-651X (ISSN-L)
- 1095-3787
- OpenAlex
- W2040008731
- Cited by
- 1,365
- References
- 1
- FWCI
- 3.25
- Type
- journal article
- Language
- en
- Open access
- bronze
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- Jarzynski, C. (1997). Equilibrium free-energy differences from nonequilibrium measurements: A master-equation approach. Physical Review E. https://doi.org/10.1103/physreve.56.5018
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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