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Temperature Dependence of the Nitrogen-Vacancy Magnetic Resonance in Diamond
Open accessAbstract
The temperature dependence of the magnetic-resonance spectra of nitrogen-vacancy (${\mathrm{NV}}^{\ensuremath{-}}$) ensembles in the range of 280--330 K was studied. Four samples prepared under different conditions were analyzed with ${\mathrm{NV}}^{\ensuremath{-}}$ concentrations ranging from 10 ppb to 15 ppm. For all samples, the axial zero-field splitting (ZFS) parameter $D$ was found to vary significantly with temperature, $T$, as $dD/dT=\ensuremath{-}74.2(7)\text{ }\text{ }\mathrm{kHz}/\mathrm{K}$. The transverse ZFS parameter $E$ was nonzero (between 4 and 11 MHz) in all samples, and exhibited a temperature dependence of $dE/(EdT)=\ensuremath{-}1.4(3)\ifmmode\times\else\texttimes\fi{}{10}^{\ensuremath{-}4}\text{ }\text{ }{\mathrm{K}}^{\ensuremath{-}1}$. The results might be accounted for by considering local thermal expansion. The temperature dependence of the ZFS parameters presents a significant challenge for diamond magnetometers and may ultimately limit their bandwidth and sensitivity.
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Cited by
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Doherty, M. W., Manson, N. B., Delaney, P., Jelezko, F., Wrachtrup, J., & Hollenberg, L. C. L. (2013) · Physics Reports · doi:10.1016/j.physrep.2013.02.001 · Cited by 2,866
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Alkauskas, A., Buckley, B. B., Awschalom, D. D., & Van de Walle, C. G. (2014) · New Journal of Physics · doi:10.1088/1367-2630/16/7/073026 · Cited by 334
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Metadata
- Authors
- Acosta, V. M., Bauch, E., Ledbetter, M. P., Waxman, A., Bouchard, L.-S., & Budker, D.
- Venue
- Physical Review Letters
- Publisher
- American Physical Society (APS)
- Published
- 2010-02-17
- Volume
- 104
- Issue
- 7
- Pages
- 070801-070801
- ISSN
- 0031-9007 (ISSN-L)
- 1079-7114
- OpenAlex
- W1995664068
- Cited by
- 735
- References
- 1
- FWCI
- 6.18
- Type
- journal article
- Language
- en
- Open access
- green
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- Acosta, V. M., Bauch, E., Ledbetter, M. P., Waxman, A., Bouchard, L.-S., & Budker, D. (2010). Temperature Dependence of the Nitrogen-Vacancy Magnetic Resonance in Diamond. Physical Review Letters. https://doi.org/10.1103/physrevlett.104.070801
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