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Spin Waves and Revised Crystal Structure of Honeycomb IridateNa2IrO3
Open accessAbstract
We report inelastic neutron scattering measurements on Na2IrO3, a candidate for the Kitaev spin model on the honeycomb lattice. We observe spin-wave excitations below 5 meV with a dispersion that can be accounted for by including substantial further-neighbor exchanges that stabilize zigzag magnetic order. The onset of long-range magnetic order below T(N)=15.3 K is confirmed via the observation of oscillations in zero-field muon-spin rotation experiments. Combining single-crystal diffraction and density functional calculations we propose a revised crystal structure model with significant departures from the ideal 90° Ir-O-Ir bonds required for dominant Kitaev exchange.
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Cites
Efficient iterative schemes for ab initio total-energy calculations using a plane-wave basis set
Kresse, G., & Furthmüller, J. (1996) · Physical Review B · doi:10.1103/physrevb.54.11169 · Cited by 123,652
Anyons in an exactly solved model and beyond
Kitaev, A. (2006) · Annals of Physics · doi:10.1016/j.aop.2005.10.005 · Cited by 5,245
Cited by
Proximate Kitaev quantum spin liquid behaviour in a honeycomb magnet
Banerjee, A., Bridges, C. A., Yan, J.-Q., Aczel, A. A., Li, L., Stone, M. B., Granroth, G. E., Lumsden, M. D., Yiu, Y., Knolle, J., et al. (2016) · Nature Materials · doi:10.1038/nmat4604 · Cited by 835
Successive magnetic phase transitions inα−RuCl3: XY-like frustrated magnet on the honeycomb lattice
Kubota, Y., Tanaka, H., Ono, T., Narumi, Y., & Kindo, K. (2015) · Physical Review B · doi:10.1103/physrevb.91.094422 · Cited by 317
Neutron tomography of magnetic Majorana fermions in a proximate quantum spin liquid
Banerjee, A., Yan, J., Knolle, J., Bridges, C. A., Stone, M. B., Lumsden, M. D., Mandrus, D. G., Tennant, D. M., Moessner, R., & Nagler, S. E. (2016) · arXiv (Cornell University) · doi:10.48550/arxiv.1609.00103 · Cited by 258
Field-induced quantum spin disordered state in spin-1/2 honeycomb magnet Na2Co2TeO6
Lin, G., Jeong, J., Kim, C., Wang, Y., Huang, Q., Masuda, T., Asai, S., Itoh, S., Günther, G., Russina, M., et al. (2021) · Nature Communications · doi:10.1038/s41467-021-25567-7 · Cited by 158
Metadata
- Authors
- Choi, S. K., Coldea, R., Kolmogorov, A. N., Lancaster, T., Mazin, I. I., Blundell, S. J., Radaelli, P. G., Singh, Y., Gegenwart, P., Choi, K. R., Cheong, S.-W., Baker, P. J., Stock, C., & Taylor, J.
- Venue
- Physical Review Letters
- Publisher
- American Physical Society (APS)
- Published
- 2012-03-20
- Volume
- 108
- Issue
- 12
- Pages
- 127204-127204
- ISSN
- 0031-9007 (ISSN-L)
- 1079-7114
- OpenAlex
- W2038928438
- Cited by
- 596
- References
- 2
- FWCI
- 28.68
- Type
- journal article
- Language
- en
- Open access
- green
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- Choi, S. K., Coldea, R., Kolmogorov, A. N., Lancaster, T., Mazin, I. I., Blundell, S. J., Radaelli, P. G., Singh, Y., Gegenwart, P., Choi, K. R., Cheong, S.-W., Baker, P. J., Stock, C., & Taylor, J. (2012). Spin Waves and Revised Crystal Structure of Honeycomb IridateNa2IrO3. Physical Review Letters. https://doi.org/10.1103/physrevlett.108.127204
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