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Attosecond Delays in Molecular Photoionization
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We report measurements of energy-dependent photoionization delays between the two outermost valence shells of N_{2}O and H_{2}O. The combination of single-shot signal referencing with the use of different metal foils to filter the attosecond pulse train enables us to extract delays from congested spectra. Remarkably large delays up to 160 as are observed in N_{2}O, whereas the delays in H_{2}O are all smaller than 50 as in the photon-energy range of 20-40 eV. These results are interpreted by developing a theory of molecular photoionization delays. The long delays measured in N_{2}O are shown to reflect the population of molecular shape resonances that trap the photoelectron for a duration of up to ∼110 as. The unstructured continua of H_{2}O result in much smaller delays at the same photon energies. Our experimental and theoretical methods make the study of molecular attosecond photoionization dynamics accessible.
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“Most recently, attosecond photoionization delays have been measured in molecules [200] and highharmonic spectroscopy has been developed further to reconstruct charge migration in spatially oriented molecules on attosecond timescales [171].”
From Roadmap of ultrafast x-ray atomic and molecular physics (2018) · cites this paper as [200]
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Zinchenko, K. S., Ardana‐Lamas, F., Lanfaloni, V. U., Luu, T. T., Pertot, Y., Huppert, M., & Wörner, H. J. (2023) · Scientific Reports · doi:10.1038/s41598-023-29089-8 · Cited by 18
Self-citationRole of nuclear-electronic coupling in attosecond photoionization of H2
Wang, A. L., Serov, V. V., Kamalov, A., Bucksbaum, P. H., Kheifets, A. S., & Cryan, J. P. (2021) · Physical Review A · doi:10.1103/physreva.104.063119 · Cited by 19
Raman time-delay in attosecond transient absorption of strong-field created krypton vacancy
Wang, L., Bai, G., Wang, X., Zhao, J., Gao, C., Wang, J., Xiao, F., Tao, W., Song, P., Qiu, Q., et al. (2024) · Nature Communications · doi:10.1038/s41467-024-47088-9 · Cited by 21
Reconstruction of Nanoscale Near Fields by Attosecond Streaking
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Probing time delays and coherent imaging of multiphoton resonant ionization
Ge, P., Han, M., Liu, M., Gong, Q., & Liu, Y. (2018) · Physical Review A · doi:10.1103/physreva.98.013409 · Cited by 19
Revealing the Target Electronic Structure with Under-Threshold RABBITT
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Time delay in XUV/IR photoionization of H2O
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Wigner time delay in photodetachment
Saha, S., Jose, J., Deshmukh, P. C., Aravind, G., Dolmatov, V. K., Kheifets, A. S., & Manson, S. T. (2019) · Physical Review A · doi:10.1103/physreva.99.043407 · Cited by 18
Controlling photoionization using attosecond time-slit interferences
Cheng, Y.-C., Mikaelsson, S., Nandi, S., Rämisch, L., Guo, C., Carlström, S., Harth, A., Vogelsang, J., Miranda, M., Arnold, C. L., et al. (2020) · Proceedings of the National Academy of Sciences · doi:10.1073/pnas.1921138117 · Cited by 15
Eisenbud–Wigner–Smith time delay in atom–laser interactions
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Coulomb focusing in attosecond angular streaking
Li, X., Liu, X., Wang, C., Ben, S., Zhou, S., Yang, Y., Song, X., Chen, J., Yang, W., & Ding, D. (2024) · Light Science & Applications · doi:10.1038/s41377-024-01600-4 · Cited by 17
Yuan, K., & Bandrauk, A. D. (2019) · Physical Chemistry Chemical Physics · doi:10.1039/c9cp05213e · Cited by 17
González‐Castrillo, A., Martı́n, F., & Palacios, A. (2020) · Scientific Reports · doi:10.1038/s41598-020-69733-1 · Cited by 17
Gregory, M., Hockett, P., Stolow, A., & Makhija, V. S. (2021) · Journal of Physics B Atomic Molecular and Optical Physics · doi:10.1088/1361-6455/ac135f · Cited by 17
Influence of nuclear dynamics on molecular attosecond photoelectron interferometry
Ertel, D., Busto, D., Makos, I., Schmoll, M., Benda, J., Ahmadi, H., Moioli, M., Frassetto, F., Poletto, L., Schröter, C. D., et al. (2023) · Science Advances · doi:10.1126/sciadv.adh7747 · Cited by 17
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Resonant photoionization of O 2 up to the fourth ionization threshold
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Attosecond spectroscopy for filming the ultrafast movies of atoms, molecules and solids
He, L., Zhu, X.-S., Cao, W., Lan, P., & Lu, P. (2022) · Chinese Physics B · doi:10.1088/1674-1056/aca6d2 · Cited by 14
Full Characterization of a Molecular Cooper Minimum Using High-Harmonic Spectroscopy
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Attosecond physics and technology
Alexander, O., Ayuso, D., Matthews, M., Rego, L., Tisch, J. W. G., Weaver, B., & Marangos, J. P. (2025) · Applied Physics Letters · doi:10.1063/5.0251524 · Cited by 18
Metadata
- Authors
- Huppert, M., Jordan, I., Baykusheva, D., von Conta, A., & Wörner, H. J.
- Affiliations
- ETH Zurich (CH)
- Venue
- Physical Review Letters
- Publisher
- American Physical Society (APS)
- Published
- 2016-08-22
- Volume
- 117
- Issue
- 9
- Pages
- 093001-093001
- ISSN
- 0031-9007 (ISSN-L)
- 1079-7114
- OpenAlex
- W2508703147
- Cited by
- 283
- References
- 45
- Citations by year
- 2026: 17 · 2025: 37 · 2024: 35 · 2023: 25 · 2022: 31 · 2021: 27 · 2020: 36 · 2019: 22 · 2018: 28 · 2017: 22 · 2016: 2
- FWCI
- 11.66
- Type
- journal article
- Language
- en
- Open access
- green
- arxiv.org
- Locations
- Physical Review Letters (publishedVersion)
- PubMed (publishedVersion)
- arXiv (Cornell University) (submittedVersion)
- arXiv (Cornell University)
- Funders
- European Research Council (307270-ATTOSCOPE)
- Schweizerischer Nationalfonds zur Förderung der Wissenschaftlichen Forschung
- NCCR-MUST
- Topics
- Physical Sciences › Physics and Astronomy › Atomic and Molecular Physics, and Optics › Laser-Matter Interactions and Applications
- Physical Sciences › Physics and Astronomy › Atomic and Molecular Physics, and Optics › Atomic and Molecular Physics
- Physical Sciences › Physics and Astronomy › Atomic and Molecular Physics, and Optics › Spectroscopy and Quantum Chemical Studies
- Keywords
- molecular photoionization, N2O, water, shape resonances, photoelectron trapping, photoionization dynamics
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