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Isotope-Induced Quantum-Phase Transitions in the Liquid State
Abstract
Isotopic binary liquid mixtures are universally characterized by an upper critical solution temperature as a consequence of zero-point motion in conjunction with the anharmonicity of the interatomic potential. This quantum effect is predicted, and demonstrated by small-angle neutron-scattering measurements, to be manifest at ambient temperatures for mixtures of deuterated and protonated polymers. Prior evidence of such phase behavior has been restricted to liquid mixtures of $^{3}\mathrm{He}$ and $^{4}\mathrm{He}$.
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Cited by
Multiblock Polymers: Panacea or Pandora’s Box?
Bates, F. S., Hillmyer, M. A., Lodge, T. P., Bates, C. M., Delaney, K. T., & Fredrickson, G. H. (2012) · Science · doi:10.1126/science.1215368 · Cited by 1,147
Self-citationGeneral Strategies for Nanoparticle Dispersion
Mackay, M. E., Tuteja, A., Duxbury, P. M., Hawker, C. J., Van Horn, B., Guan, Z., Chen, G., & Krishnan, R. S. (2006) · Science · doi:10.1126/science.1122225 · Cited by 960
Spinodal decomposition of a symmetric critical mixture of deuterated and protonated polymer
Bates, F. S., & Wiltzius, P. (1989) · The Journal of Chemical Physics · doi:10.1063/1.456901 · Cited by 388
Self-citationSurface Enrichment in an Isotopic Polymer Blend
Jones, R. A. L., Kramer, E. J., Rafailovich, M. H., Sokolov, J., & Schwarz, S. A. (1989) · Physical Review Letters · doi:10.1103/physrevlett.62.280 · Cited by 269
Metadata
- Authors
- Bates, F. S., & Wignall, G. D.
- Venue
- Physical Review Letters
- Publisher
- American Physical Society (APS)
- Published
- 1986-09-22
- Volume
- 57
- Issue
- 12
- Pages
- 1429-1432
- ISSN
- 0031-9007 (ISSN-L)
- OpenAlex
- W2005147892
- Cited by
- 162
- References
- 0
- FWCI
- 8.99
- Type
- journal article
- Language
- en
- Open access
- closed
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