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Room Temperature Polariton Emission from Strongly Coupled Organic Semiconductor Microcavities
Abstract
We report a room temperature study of the strong exciton-photon coupling regime in a planar microcavity, containing cyanine dye aggregates with delocalized exciton wave functions ( $J$ aggregates). Giant Rabi splittings of 80 meV between upper and lower polariton branches are observed and cavity polariton emission is detected from the lower polariton branch. The small linewidth and large oscillator strength characteristic of $J$ aggregates make them a favorable physical structure to allow the observation of strong coupling for organic semiconductors.
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Cited by
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Törmä, P., & Barnes, W. L. (2015) · Reports on Progress in Physics · doi:10.1088/0034-4885/78/1/013901 · Cited by 1,644
Room-Temperature Bose–Einstein Condensation of Cavity Exciton–Polaritons in a Polymer
Plumhof, J. D., Stöferle, T., Mai, L., Scherf, U., & Mahrt, R. F. (2014) · Nature Materials · doi:10.1038/nmat3825 · Cited by 745
Reversible Switching of Ultrastrong Light-Molecule Coupling
Schwartz, T., Hutchison, J. A., Genet, C., & Ebbesen, T. W. (2011) · Physical Review Letters · doi:10.1103/physrevlett.106.196405 · Cited by 658
Polariton-Mediated Energy Transfer between Organic Dyes in a Strongly Coupled Optical Microcavity
Coles, D. M., Somaschi, N., Michetti, P., Clark, C., Lagoudakis, P. G., Savvidis, P. G., & Lidzey, D. G. (2014) · Nature Materials · doi:10.1038/nmat3950 · Cited by 507
Strong light–matter interactions: a new direction within chemistry
Hertzog, M., Wang, M., Mony, J., & Börjesson, K. (2019) · Chemical Society Reviews · doi:10.1039/c8cs00193f · Cited by 444
Metadata
- Authors
- Lidzey, D. G., Bradley, D. D. C., Virgili, T., Armitage, A., Skolnick, M. S., & Walker, S.
- Venue
- Physical Review Letters
- Publisher
- American Physical Society (APS)
- Published
- 1999-04-19
- Volume
- 82
- Issue
- 16
- Pages
- 3316-3319
- ISSN
- 0031-9007 (ISSN-L)
- 1079-7114
- OpenAlex
- W2048621757
- Cited by
- 385
- References
- 0
- FWCI
- 8.98
- Type
- journal article
- Language
- en
- Open access
- closed
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- Lidzey, D. G., Bradley, D. D. C., Virgili, T., Armitage, A., Skolnick, M. S., & Walker, S. (1999). Room Temperature Polariton Emission from Strongly Coupled Organic Semiconductor Microcavities. Physical Review Letters. https://doi.org/10.1103/physrevlett.82.3316
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