The DOI matches its Crossref record; 34 of the 34 references it cites were found in a registry or an index.
Reversible Switching of Ultrastrong Light-Molecule Coupling
Abstract
We demonstrate that photochromic molecules enable switching from the weak- to ultrastrong-coupling regime reversibly, by using all-optical control. This switch is achieved by photochemically inducing conformational changes in the molecule. Remarkably, a Rabi splitting of 700 meV is measured at room temperature, corresponding to 32% of the molecular transition energy. A similar coupling strength is demonstrated in a plasmonic structure. Such systems present a unique combination of coupling strength and functional capacities.
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Cited by
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Nonlinear optical signals and spectroscopy with quantum light
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Theoretical Advances in Polariton Chemistry and Molecular Cavity Quantum Electrodynamics
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Virtual photons in the ground state of a dissipative system
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Metadata
- Authors
- Schwartz, T., Hutchison, J. A., Genet, C., & Ebbesen, T. W.
- Venue
- Physical Review Letters
- Publisher
- American Physical Society (APS)
- Published
- 2011-05-11
- Volume
- 106
- Issue
- 19
- Pages
- 196405-196405
- ISSN
- 0031-9007 (ISSN-L)
- 1079-7114
- OpenAlex
- W2054838521
- Cited by
- 658
- References
- 34
- FWCI
- 19.46
- Type
- journal article
- Language
- en
- Open access
- closed
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