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Nonclassical Photon Statistics in Single-Molecule Fluorescence at Room Temperature
Abstract
The fluorescence of single terrylene molecules in a crystalline host is investigated at room temperature by scanning confocal optical microscopy. Photon arrival times are analyzed in terms of interphoton time distributions, second order correlation functions, and the variance of the photon number probability distribution. Antibunching at short times and bunching behavior for longer times is observed, associated with sub- and super-Poissonian statistics, respectively. A rate-equation analysis of the molecular level populations indicates an accelerated reverse intersystem crossing.
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Citations
Cited by
Gisin, N., Ribordy, G., Tittel, W., & Zbinden, H. (2002) · Reviews of Modern Physics · doi:10.1103/revmodphys.74.145 · Cited by 8,515
Invited Review Article: Single-photon sources and detectors
Eisaman, M. D., Fan, J., Migdall, A., & Polyakov, S. V. (2011) · Review of Scientific Instruments · doi:10.1063/1.3610677 · Cited by 1,358
Quantum correlation among photons from a single quantum dot at room temperature
Michler, P., Imamoğlu, A., Mason, M. D., Carson, P. J., Strouse, G. F., & Buratto, S. K. (2000) · Nature · doi:10.1038/35023100 · Cited by 964
Lounis, B., & Orrit, M. (2005) · Reports on Progress in Physics · doi:10.1088/0034-4885/68/5/r04 · Cited by 908
Nonlinear optical signals and spectroscopy with quantum light
Dorfman, K. E., Schlawin, F., & Mukamel, S. (2016) · Reviews of Modern Physics · doi:10.1103/revmodphys.88.045008 · Cited by 361
Metadata
- Authors
- Fleury, L., Segura, J.-M., Zumofen, G., Hecht, B., & Wild, U. P.
- Venue
- Physical Review Letters
- Publisher
- American Physical Society (APS)
- Published
- 2000-02-07
- Volume
- 84
- Issue
- 6
- Pages
- 1148-1151
- ISSN
- 0031-9007 (ISSN-L)
- 1079-7114
- OpenAlex
- W2044213208
- Cited by
- 253
- References
- 0
- FWCI
- 12.56
- Type
- journal article
- Language
- en
- Open access
- closed
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- Fleury, L., Segura, J.-M., Zumofen, G., Hecht, B., & Wild, U. P. (2000). Nonclassical Photon Statistics in Single-Molecule Fluorescence at Room Temperature. Physical Review Letters. https://doi.org/10.1103/physrevlett.84.1148
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