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Double Resonant Raman Scattering in Graphite
Abstract
We find that the electronic dispersion in graphite gives rise to double resonant Raman scattering for excitation energies up to 5 eV. As we show, the curious excitation-energy dependence of the graphite D mode is due to this double resonant process resolving a long-standing problem in the literature and invalidating recent attempts to explain this phenomenon. Our calculation for the D-mode frequency shift ( 60 cm(-1)/eV) agrees well with the experimental value.
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Citations
Cited by
Raman spectroscopy as a versatile tool for studying the properties of graphene
Ferrari, A. C., & Basko, D. M. (2013) · Nature Nanotechnology · doi:10.1038/nnano.2013.46 · Cited by 7,405
Chemical oxidation of multiwalled carbon nanotubes
Datsyuk, V., Kalyva, M., Papagelis, K., Parthenios, J., Tasis, D., Siokou, A., Kallitsis, I., & Galiotis, C. (2008) · Carbon · doi:10.1016/j.carbon.2008.02.012 · Cited by 2,747
Raman spectroscopy of graphite
Reich, S., & Thomsen, C. (2004) · Philosophical Transactions of the Royal Society of London. Series A: Mathematical, Physical and Engineering Sciences · doi:10.1098/rsta.2004.1454 · Cited by 1,312
Self-citationGouadec, G., & Colomban, P. (2007) · Progress in Crystal Growth and Characterization of Materials · doi:10.1016/j.pcrysgrow.2007.01.001 · Cited by 1,050
Influence of the Atomic Structure on the Raman Spectra of Graphite Edges
Cançado, L. G., Pimenta, M. A., Neves, B. R. A., Dantas, M. S. S., & Jorio, A. (2004) · Physical Review Letters · doi:10.1103/physrevlett.93.247401 · Cited by 668
Metadata
- Authors
- Thomsen, C., & Reich, S.
- Venue
- Physical Review Letters
- Publisher
- American Physical Society (APS)
- Published
- 2000-12-11
- Volume
- 85
- Issue
- 24
- Pages
- 5214-5217
- ISSN
- 0031-9007 (ISSN-L)
- 1079-7114
- OpenAlex
- W2082174079
- Cited by
- 1,773
- References
- 0
- FWCI
- 19.26
- Type
- journal article
- Language
- en
- Open access
- closed
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