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Rapid Transport of Gases in Carbon Nanotubes
Abstract
We report atomistic simulations for both self- and transport diffusivities of light gases in carbon nanotubes and in two zeolites with comparable pore sizes. We find that transport rates in nanotubes are orders of magnitude faster than in the zeolites we have studied or in any microporous material for which experimental data are available. The exceptionally high transport rates in nanotubes are shown to be a result of the inherent smoothness of the nanotubes. We predict that carbon nanotube membranes will have fluxes that are orders of magnitude greater than crystalline zeolite membranes.
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Citations
Cited by
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Chen, X. Y., Vinh-Thang, H., Ramirez, A. A., Rodrigue, D., & Kaliaguine, S. (2015) · RSC Advances · doi:10.1039/c5ra00666j · Cited by 503
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Metadata
- Authors
- Skoulidas, A. I., Ackerman, D. M., Johnson, J. K., & Sholl, D. S.
- Venue
- Physical Review Letters
- Publisher
- American Physical Society (APS)
- Published
- 2002-10-14
- Volume
- 89
- Issue
- 18
- Pages
- 185901-185901
- ISSN
- 0031-9007 (ISSN-L)
- 1079-7114
- OpenAlex
- W2086965189
- Cited by
- 690
- References
- 0
- FWCI
- 74.22
- Type
- journal article
- Language
- en
- Open access
- closed
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- Skoulidas, A. I., Ackerman, D. M., Johnson, J. K., & Sholl, D. S. (2002). Rapid Transport of Gases in Carbon Nanotubes. Physical Review Letters. https://doi.org/10.1103/physrevlett.89.185901
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
Semantic Scholar’s data is described in: Kinney, R., et al. (2023). The Semantic Scholar Open Data Platform. arXiv:2301.10140.