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Ultrafast Optical Switching to a Metallic State by Photoinduced Mott Transition in a Halogen-Bridged Nickel-Chain Compound
Open accessAbstract
We demonstrate the ultrafast photoinduced Mott transition from a charge transfer insulator to a metal in a halogen-bridged Ni-chain compound by pump-probe reflection spectroscopy. Upon the irradiation of a 130-femtosecond laser pulse, the spectral weight of the gap transition is transferred to the inner-gap region. When the photoexcitation density exceeds 0.1/Ni site, the Drude-like high-reflection band appears in the infrared region, signaling the formation of a metallic state. The photogeneration of the metallic state and the subsequent recovery to the original gapped state occur within a few picoseconds.
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Self-citationOrbital Physics in Transition-Metal Oxides
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Self-citationOptical spectra ofLa2−xSrxCuO4: Effect of carrier doping on the electronic structure of theCuO2plane
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Self-citationGigantic optical nonlinearity in one-dimensional Mott–Hubbard insulators
Kishida, H., Matsuzaki, H., Okamoto, H., Manabe, T., Yamashita, M., Taguchi, Y., & Tokura, Y. (2000) · Nature · doi:10.1038/35016036 · Cited by 356
Self-citationSingularities in Optical Spectra of Quantum Spin Chains
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Self-citationYu, G., Lee, C., Heeger, A. J., et al. (1991) · Physical Review Letters · doi:10.1103/physrevlett.67.2581 · Cited by 108
Midinfrared optical excitations in undoped lamellar copper oxides
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One-dimensional cuprate as a nonlinear optical material for ultrafast all-optical switching
Ashida, M., Ogasawara, T., Tokura, Y., Uchida, S., Mazumdar, S., & Kuwata‐Gonokami, M. (2001) · Applied Physics Letters · doi:10.1063/1.1370546 · Cited by 39
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Floquet Engineering of Quantum Materials
Oka, T., & Kitamura, S. (2019) · Annual Review of Condensed Matter Physics · doi:10.1146/annurev-conmatphys-031218-013423 · Cited by 999
Nonequilibrium dynamical mean-field theory and its applications
Aoki, H., Tsuji, N., Eckstein, M., Kollar, M., Oka, T., & Werner, P. (2014) · Reviews of Modern Physics · doi:10.1103/revmodphys.86.779 · Cited by 773
Metadata
- Authors
- Iwai, S., Ono, M., Maeda, A., Matsuzaki, H., Kishida, H., Okamoto, H., & Tokura, Y.
- Venue
- Physical Review Letters
- Publisher
- American Physical Society (APS)
- Published
- 2003-07-28
- Volume
- 91
- Issue
- 5
- Pages
- 057401-057401
- ISSN
- 0031-9007 (ISSN-L)
- 1079-7114
- OpenAlex
- W2080045732
- Cited by
- 334
- References
- 8
- FWCI
- 7.96
- Type
- journal article
- Language
- en
- Open access
- green
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- Iwai, S., Ono, M., Maeda, A., Matsuzaki, H., Kishida, H., Okamoto, H., & Tokura, Y. (2003). Ultrafast Optical Switching to a Metallic State by Photoinduced Mott Transition in a Halogen-Bridged Nickel-Chain Compound. Physical Review Letters. https://doi.org/10.1103/physrevlett.91.057401
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