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Space-Charge Limited Photocurrent
Open accessAbstract
In 1971 Goodman and Rose predicted the occurrence of a fundamental electrostatic limit for the photocurrent in semiconductors at high light intensities. Blends of conjugated polymers and fullerenes are an ideal model system to observe this space-charge limit experimentally, since they combine an unbalanced charge transport, long lifetimes, high charge carrier generation efficiencies, and low mobility of the slowest charge carrier. The experimental photocurrents reveal all the characteristics of a space-charge limited photocurrent: a one-half power dependence on voltage, a three-quarter power dependence on light intensity, and a one-half power scaling of the voltage at which the photocurrent switches into full saturation with light intensity.
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Citations
Cited by
He, Z., Zhong, C., Huang, X., Wong, W., Wu, H., Chen, L., Su, S., & Cao, Y. (2011) · Advanced Materials · doi:10.1002/adma.201103006 · Cited by 2,134
Mihailetchi, V. D., Xie, H. X., de Boer, B., Koster, L. J. A., & Blom, P. W. M. (2006) · Advanced Functional Materials · doi:10.1002/adfm.200500420 · Cited by 1,283
Self-citationCharacterization of nanostructured hybrid and organic solar cells by impedance spectroscopy
Fabregat-Santiago, F., Garcia-Belmonte, G., Mora-Seró, I., & Bisquert, J. (2011) · Physical Chemistry Chemical Physics · doi:10.1039/c0cp02249g · Cited by 1,206
Dual Plasmonic Nanostructures for High Performance Inverted Organic Solar Cells
Li, X., Choy, W. C. H., Huo, L., Xie, F., Sha, W. E. I., Ding, B., Guo, X., Li, Y., Hou, J., You, J., et al. (2012) · Advanced Materials · doi:10.1002/adma.201200120 · Cited by 699
Hole Selective NiO Contact for Efficient Perovskite Solar Cells with Carbon Electrode
Xu, X., Liu, Z., Zuo, Z., Zhang, M., Zhao, Z., Shen, Y., Zhou, H., Chen, Q., Yang, Y., & Wang, M. (2015) · Nano Letters · doi:10.1021/nl504701y · Cited by 445
Metadata
- Authors
- Mihailetchi, V. D., Wildeman, J., & Blom, P. W. M.
- Venue
- Physical Review Letters
- Publisher
- American Physical Society (APS)
- Published
- 2005-04-01
- Volume
- 94
- Issue
- 12
- Pages
- 126602-126602
- ISSN
- 0031-9007 (ISSN-L)
- 1079-7114
- OpenAlex
- W2102124889
- Cited by
- 1,130
- References
- 0
- FWCI
- 20.34
- Type
- journal article
- Language
- en
- Open access
- green
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