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OrthorhombicFdddNetwork in Triblock and Diblock Copolymer Melts
Abstract
The phase behavior of ABC triblock and AB diblock copolymer melts is investigated by self-consistent field theory, while allowing for (among other candidates) the orthorhombic Fddd (O70) network phase identified in recent experiments with poly(isoprene-b-styrene-b-ethylene oxide) (ISO) triblocks. Predicted phase diagrams for triblocks similar to ISO contain an O70 phase bordered by gyroid, lamellar, and alternating gyroid phases, in agreement with experiment. The O70 network is also found to be stable in diblock melts within a narrow region that overlaps the weak segregation end of the gyroid region found in previous calculations.
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Citations
Cited by
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Bates, C. M., & Bates, F. S. (2017) · Macromolecules · doi:10.1021/acs.macromol.6b02355 · Cited by 788
Polydispersity and block copolymer self-assembly
Lynd, N. A., Meuler, A. J., & Hillmyer, M. A. (2008) · Progress in Polymer Science · doi:10.1016/j.progpolymsci.2008.07.003 · Cited by 485
Discovering ordered phases of block copolymers: New results from a generic fourier-space approach
Guo, Z., Zhang, G., Qiu, F., Zhang, H., Yang, Y., & Shi, A.-C. (2008) · Physical Review Letters · doi:10.1103/physrevlett.101.028301 · Cited by 150
The Block Copolymer Phase Behavior Database
Rebello, N. J., Arora, A., Mochigase, H., Lin, T.-S., Shi, J., Audus, D. J., Muckley, E. S., Osmani, A., & Olsen, B. D. (2024) · Journal of Chemical Information and Modeling · doi:10.1021/acs.jcim.4c00242 · Cited by 12
Metadata
- Authors
- Tyler, C. A., & Morse, D. C.
- Venue
- Physical Review Letters
- Publisher
- American Physical Society (APS)
- Published
- 2005-05-24
- Volume
- 94
- Issue
- 20
- Pages
- 208302-208302
- ISSN
- 0031-9007 (ISSN-L)
- 1079-7114
- OpenAlex
- W2028079037
- Cited by
- 308
- References
- 0
- FWCI
- 7.46
- Type
- journal article
- Language
- en
- Open access
- closed
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