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Gold-Adatom-Mediated Bonding in Self-Assembled Short-Chain Alkanethiolate Species on the Au(111) Surface
Abstract
Microscopic evidence for Au-adatom-induced self-assembly of alkanethiolate species on the Au(111) surface is presented. Based on STM measurements and density-functional theory calculations, a new model for the low-coverage self-assembled monolayer of alkanethiolate on the Au(111) surface is developed, which involves the adsorbate complexes incorporating Au adatoms. It is also concluded that the Au(111) herringbone reconstruction is lifted by the alkanethiolate self-assembly because the reconstructed surface layer provides reactive Au adatoms that drive self-assembly.
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Projector augmented-wave method
Blöchl, P. E. (1994) · Physical Review B · doi:10.1103/physrevb.50.17953 · Cited by 92,732
From ultrasoft pseudopotentials to the projector augmented-wave method
Kresse, G., & Joubert, D. (1999) · Physical Review B · doi:10.1103/physrevb.59.1758 · Cited by 85,307
Special points for Brillouin-zone integrations
Monkhorst, H. J., & Pack, J. D. (1976) · Physical Review B · doi:10.1103/physrevb.13.5188 · Cited by 71,721
Cited by
A unified view of ligand-protected gold clusters as superatom complexes
Walter, M., Akola, J., Lopez-Acevedo, O., Jadzinsky, P. D., Calero, G., Ackerson, C. J., Whetten, R. L., Grönbeck, H., & Häkkinen, H. (2008) · Proceedings of the National Academy of Sciences · doi:10.1073/pnas.0801001105 · Cited by 1,742
Chaki, N. K., Negishi, Y., Tsunoyama, H., Shichibu, Y., & Tsukuda, T. (2008) · Journal of the American Chemical Society · doi:10.1021/ja8005379 · Cited by 393
Zhukhovitskiy, A. V., MacLeod, M. J., & Johnson, J. A. (2015) · Chemical Reviews · doi:10.1021/acs.chemrev.5b00220 · Cited by 363
Properties of the gold–sulphur interface: from self-assembled monolayers to clusters
Bürgi, T. (2015) · Nanoscale · doi:10.1039/c5nr03497c · Cited by 287
Metadata
- Authors
- Maksymovych, P., Sorescu, D. C., & Yates, J. T.
- Venue
- Physical Review Letters
- Publisher
- American Physical Society (APS)
- Published
- 2006-10-06
- Volume
- 97
- Issue
- 14
- Pages
- 146103-146103
- ISSN
- 0031-9007 (ISSN-L)
- 1079-7114
- OpenAlex
- W1974436039
- Cited by
- 457
- References
- 3
- FWCI
- 24.62
- Type
- journal article
- Language
- en
- Open access
- closed
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- Maksymovych, P., Sorescu, D. C., & Yates, J. T. (2006). Gold-Adatom-Mediated Bonding in Self-Assembled Short-Chain Alkanethiolate Species on the Au(111) Surface. Physical Review Letters. https://doi.org/10.1103/physrevlett.97.146103
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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