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Quantum Magnetism in the Paratacamite Family: Towards an Ideal Kagomé Lattice
Open accessAbstract
We report muon spin rotation measurements on the $S=1/2$ (${\mathrm{Cu}}^{2+}$) paratacamite ${\mathrm{Zn}}_{x}{\mathrm{Cu}}_{4\ensuremath{-}x}(\mathrm{OH}{)}_{6}{\mathrm{Cl}}_{2}$ family. Despite a Weiss temperature of $\ensuremath{\sim}\ensuremath{-}300\text{ }\text{ }\mathrm{K}$, the $x=1$ compound is found to have no transition to a magnetic frozen state down to 50 mK as theoretically expected for the kagom\'e Heisenberg antiferromagnet. We find that the limit between a dynamical and a partly frozen ground state occurs around $x=0.5$. For $x=1$, we discuss the relevance to a singlet picture.
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Cites
Resonating valence bonds: A new kind of insulator?
Anderson, P. W. (1973) · Materials Research Bulletin · doi:10.1016/0025-5408(73)90167-0 · Cited by 2,823
(2005) · WORLD SCIENTIFIC eBooks · doi:10.1142/9789812567819 · Cited by 686
Cooperative Paramagnetism in the Geometrically Frustrated Pyrochlore AntiferromagnetTb2Ti2O7
Gardner, J. S., Dunsiger, S. R., Gaulin, B. D., Gingras, M. J. P., Greedan, J. E., Kiefl, R. F., Lumsden, M. D., MacFarlane, W. A., Raju, N. P., Sonier, J. E., et al. (1999) · Physical Review Letters · doi:10.1103/physrevlett.82.1012 · Cited by 516
Pyrochlore Antiferromagnet: A Three-Dimensional Quantum Spin Liquid
Canals, B., & Lacroix, C. (1998) · Physical Review Letters · doi:10.1103/physrevlett.80.2933 · Cited by 380
Lecheminant, P., Bernu, B., Lhuillier, C., Pierre, L., & Sindzingre, P. (1997) · Physical Review B · doi:10.1103/physrevb.56.2521 · Cited by 362
Spin-1/2 Kagomé-Like Lattice in Volborthite Cu3V2O7(OH)2·2H2O
Hiroi, Z., Hanawa, M., Kobayashi, N., Nohara, M., Takagi, H., Kato, Y., & Takigawa, M. (2001) · Journal of the Physical Society of Japan · doi:10.1143/jpsj.70.3377 · Cited by 256
Low-Energy Sector of theS=1/2Kagome Antiferromagnet
Mila, F. (1998) · Physical Review Letters · doi:10.1103/physrevlett.81.2356 · Cited by 245
Cited by
Spin liquids in frustrated magnets
Balents, L. (2010) · Nature · doi:10.1038/nature08917 · Cited by 4,316
Colloquium : Herbertsmithite and the search for the quantum spin liquid
Norman, M. R. (2016) · Reviews of Modern Physics · doi:10.1103/revmodphys.88.041002 · Cited by 580
Metadata
- Authors
- Mendels, P., Bert, F., de Vries, M. A., Olariu, A., Harrison, A., Duc, F., Trombe, J. C., Lord, J. S., Amato, A., & Baines, C.
- Venue
- Physical Review Letters
- Publisher
- American Physical Society (APS)
- Published
- 2007-02-13
- Volume
- 98
- Issue
- 7
- Pages
- 077204-077204
- ISSN
- 0031-9007 (ISSN-L)
- 1079-7114
- OpenAlex
- W2006235853
- Cited by
- 465
- References
- 7
- FWCI
- 32.45
- Type
- journal article
- Language
- en
- Open access
- bronze
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- Mendels, P., Bert, F., de Vries, M. A., Olariu, A., Harrison, A., Duc, F., Trombe, J. C., Lord, J. S., Amato, A., & Baines, C. (2007). Quantum Magnetism in the Paratacamite Family: Towards an Ideal Kagomé Lattice. Physical Review Letters. https://doi.org/10.1103/physrevlett.98.077204
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