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Phonon Anharmonicities in Graphite and Graphene
Open accessAbstract
We determine from first principles the finite-temperature properties-linewidths, line shifts, and lifetimes-of the key vibrational modes that dominate inelastic losses in graphitic materials. In graphite, the phonon linewidth of the Raman-active E(2g) mode is found to decrease with temperature; such anomalous behavior is driven entirely by electron-phonon interactions, and does not appear in the nearly degenerate infrared-active E(1u) mode. In graphene, the phonon anharmonic lifetimes and decay channels of the A(1)' mode at K dominate over E(2g) at Gamma and couple strongly with acoustic phonons, highlighting how ballistic transport in carbon-based interconnects requires careful engineering of phonon decays and thermalization.
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Citations
Cites
High-field electrical transport in single-wall carbon nanotubes
Yao, Z., Kane, C. L., & Dekker, C. (2000) · Physical Review Letters · doi:10.1103/physrevlett.84.2941 · Cited by 1,501
Cited by
The electronic properties of graphene
Castro Neto, A. H., Guinea, F., Peres, N. M. R., Novoselov, K. S., & Geim, A. K. (2009) · Reviews of Modern Physics · doi:10.1103/revmodphys.81.109 · Cited by 24,803
“Non-linear effects such as large bending deformations (Peliti and Leibler, 1985), the coupling between flexural and in-plane modes (or phonon-phonon interactions (Bonini et al., 2007)) and the presence of topological defects (Nelson, D.”
BackgroundRaman spectroscopy as a versatile tool for studying the properties of graphene
Ferrari, A. C., & Basko, D. M. (2013) · Nature Nanotechnology · doi:10.1038/nnano.2013.46 · Cited by 7,405
Raman spectroscopy of graphene-based materials and its applications in related devices
Wu, J.-B., Lin, M.-L., Cong, X., Liu, H.-N., & Tan, P.-H. (2018) · Chemical Society Reviews · doi:10.1039/c6cs00915h · Cited by 2,092
Electron-phonon interactions from first principles
Giustino, F. (2017) · Reviews of Modern Physics · doi:10.1103/revmodphys.89.015003 · Cited by 1,604
Transfer of CVD-Grown Monolayer Graphene onto Arbitrary Substrates
Suk, J. W., Kitt, A., Magnuson, C. W., Hao, Y., Ahmed, S., An, J., Swan, A. K., Goldberg, B. B., & Ruoff, R. S. (2011) · ACS Nano · doi:10.1021/nn201207c · Cited by 1,495
Metadata
- Authors
- Bonini, N., Lazzeri, M., Marzari, N., & Mauri, F.
- Venue
- Physical Review Letters
- Publisher
- American Physical Society (APS)
- Published
- 2007-10-24
- Volume
- 99
- Issue
- 17
- Pages
- 176802-176802
- ISSN
- 0031-9007 (ISSN-L)
- 1079-7114
- OpenAlex
- W2003365324
- Cited by
- 480
- References
- 1
- FWCI
- 9.14
- Type
- journal article
- Language
- en
- Open access
- green
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- Bonini, N., Lazzeri, M., Marzari, N., & Mauri, F. (2007). Phonon Anharmonicities in Graphite and Graphene. Physical Review Letters. https://doi.org/10.1103/physrevlett.99.176802
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