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Soft-X-ray ARPES facility at the ADRESS beamline of the SLS: concepts, technical realisation and scientific applications
Open accessAbstract
Soft-X-ray angle-resolved photoelectron spectroscopy (ARPES) with photon energies around 1 keV combines the momentum space resolution with increasing probing depth. The concepts and technical realisation of the new soft-X-ray ARPES endstation at the ADRESS beamline of SLS are described. The experimental geometry of the endstation is characterized by grazing X-ray incidence on the sample to increase the photoyield and vertical orientation of the measurement plane. The vacuum chambers adopt a radial layout allowing most efficient sample transfer. High accuracy of the angular resolution is ensured by alignment strategies focused on precise matching of the X-ray beam and optical axis of the analyzer. The high photon flux of up to 10 13 photons s−1(0.01% bandwidth)−1 delivered by the beamline combined with the optimized experimental geometry break through the dramatic loss of the valence band photoexcitation cross section at soft-X-ray energies. ARPES images with energy resolution up to a few tens of meV are typically acquired on the time scale of minutes. A few application examples illustrate the power of our advanced soft-X-ray ARPES instrumentation to explore the electronic structure of bulk crystals with resolution in three-dimensional momentum, access buried heterostructures and study elemental composition of the valence states using resonant excitation.
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Lev, L. L., Averyanov, D. V., Tokmachev, A. M., Bisti, F., Rogalev, V. A., Strocov, V. N., & Storchak, V. G. (2016) · Journal of Materials Chemistry C · doi:10.1039/c6tc03737b · Cited by 41
Self-citationXu, N., Autès, G., Matt, C. E., Lv, B., Yao, M. Y., Bisti, F., Strocov, V. N., Gawryluk, D. J., Pomjakushina, E. V., Conder, K., et al. (2017) · Physical Review Letters · doi:10.1103/physrevlett.118.106406 · Cited by 40
Self-citationKrieger, J. A., Chang, C., Huşanu, M. A., Sostina, D., Ernst, A., Otrokov, M. M., Prokscha, T., Schmitt, T., Suter, A., Vergniory, M. G., et al. (2017) · Physical review. B./Physical review. B · doi:10.1103/physrevb.96.184402 · Cited by 39
Self-citationWeber, F., Hott, R., Heid, R., Lev, L. L., Caputo, M., Schmitt, T., & Strocov, V. N. (2018) · Physical review. B./Physical review. B · doi:10.1103/physrevb.97.235122 · Cited by 37
Self-citationYang, S., Schröter, N. B. M., Strocov, V. N., Schuwalow, S., Rajpalk, M., Ohtani, K., Krogstrup, P., Winkler, G. W., Gukelberger, J., Gresch, D., et al. (2022) · Advanced Quantum Technologies · doi:10.1002/qute.202100033 · Cited by 35
Self-citationBisti, F., Rogalev, V. A., Karolak, M., Paul, S., Gupta, A., Schmitt, T., Guntherodt, G., Eyert, V., Sangiovanni, G., Profeta, G., et al. (2017) · Physical Review X · doi:10.1103/physrevx.7.041067 · Cited by 34
Self-citationLiu, Y., Luchini, A., Martí‐Sánchez, S., Koch, C., Schuwalow, S., Khan, S. A., Stankevič, T., Francoual, S., Mardegan, J. R. L., Krieger, J. A., et al. (2019) · ACS Applied Materials & Interfaces · doi:10.1021/acsami.9b15034 · Cited by 34
Self-citationTrivial topological phase of CaAgP and the topological nodal-line transition in CaAg(P1−xAsx)
Xu, N., Qian, Y., Wu, Q., Autès, G., Matt, C. E., Lv, B., Yao, M. Y., Strocov, V. N., Pomjakushina, E. V., Conder, K., et al. (2018) · Physical review. B./Physical review. B · doi:10.1103/physrevb.97.161111 · Cited by 33
Self-citationControllable orbital angular momentum monopoles in chiral topological semimetals
Yen, Y., Krieger, J. A., Yao, M., Robredo, I., Manna, K., Yang, Q., McFarlane, E. C., Shekhar, C., Borrmann, H., Stolz, S., et al. (2024) · Nature Physics · doi:10.1038/s41567-024-02655-1 · Cited by 30
Self-citationElectron-polaron dichotomy of charge carriers in perovskite oxides
Husanu, M.-A., Vistoli, L., Verdi, C., Sander, A., Garcia, V., Rault, J. E., Bisti, F., Lev, L. L., Schmitt, T., Giustino, F., et al. (2020) · Communications Physics · doi:10.1038/s42005-020-0330-6 · Cited by 30
Self-citationk-resolved electronic structure of buried heterostructure and impurity systems by soft-X-ray ARPES
Strocov, V. N., Lev, L. L., Kobayashi, M., Cancellieri, C., Huşanu, M. A., Chikina, A., Schröter, N. B. M., Wang, X., Krieger, J. A., & Salman, Z. (2019) · Journal of Electron Spectroscopy and Related Phenomena · doi:10.1016/j.elspec.2019.06.009 · Cited by 30
Self-citationStable sub-micrometre high-flux probe for soft X-ray ARPES using a monolithic Wolter mirror
Senba, Y., Kishimoto, H., Takeo, Y., Yumoto, H., Koyama, T., Mimura, H., & Ohashi, H. (2020) · Journal of Synchrotron Radiation · doi:10.1107/s1600577520007274 · Cited by 29
Observation of a linked-loop quantum state in a topological magnet
Belopolski, I., Chang, G., Cochran, T. A., Cheng, Z., Yáng, X., Hugelmeyer, C., Manna, K., Yin, J., Cheng, G., Multer, D., et al. (2022) · Nature · doi:10.1038/s41586-022-04512-8 · Cited by 29
Self-citationDo topology and ferromagnetism cooperate at the EuS/Bi2Se3 interface?
Krieger, J. A., Ou, Y., Caputo, M., Chikina, A., Döbeli, M., Huşanu, M. A., Keren, I., Prokscha, T., Suter, A., Chang, C., et al. (2019) · Physical review. B./Physical review. B · doi:10.1103/physrevb.99.064423 · Cited by 28
Self-citationOrientation-dependent electronic structure in interfacial superconductors LaAlO3/KTaO3
Chen, X., Yu, T., Liu, Y., Sun, Y., Lei, M., Guo, N., Fan, Y., Sun, X., Zhang, M., Alarab, F., et al. (2024) · Nature Communications · doi:10.1038/s41467-024-51969-4 · Cited by 28
Self-citationNéel Vector Induced Manipulation of Valence States in the Collinear Antiferromagnet Mn2Au
Elmers, H. J., Chernov, S., D'Souza, S. W., Bommanaboyena, S. P., Bodnar, S., Medjanik, K., Babenkov, S., Fedchenko, O., Vasilyev, D., Ágústsson, S. Ý., et al. (2020) · ACS Nano · doi:10.1021/acsnano.0c08215 · Cited by 28
Self-citationHigh-energy photoemission final states beyond the free-electron approximation
Strocov, V. N., Lev, L. L., Alarab, F., Constantinou, P., Wang, X., Schmitt, T., Stock, T. J. Z., Nicolaï, L., Očenášek, J., & Minář, J. (2023) · Nature Communications · doi:10.1038/s41467-023-40432-5 · Cited by 27
Self-citationElectronic phase separation at LaAlO3/SrTiO3 interfaces tunable by oxygen deficiency
Strocov, V. N., Chikina, A., Caputo, M., Husanu, M.-A., Bisti, F., Bracher, D., Schmitt, T., Granozio, F. M., Vaz, C. A. F., & Lechermann, F. (2019) · Physical Review Materials · doi:10.1103/physrevmaterials.3.106001 · Cited by 27
Self-citationBand-Order Anomaly at the γ-Al2O3/SrTiO3 Interface Drives the Electron-Mobility Boost
Chikina, A., Christensen, D. V., Borisov, V., Huşanu, M. A., Chen, Y., Wang, X., Schmitt, T., Radovic, M., Nagaosa, N., Mishchenko, A. S., et al. (2021) · ACS Nano · doi:10.1021/acsnano.0c07609 · Cited by 26
Self-citationBand structure of overdoped cuprate superconductors: Density functional theory matching experiments
Kramer, K. P., Horio, M., Tsirkin, S. S., Sassa, Y., Hauser, K., Matt, C. E., Sutter, D., Chikina, A., Schröter, N. B. M., Krieger, J. A., et al. (2019) · Physical review. B./Physical review. B · doi:10.1103/physrevb.99.224509 · Cited by 26
Self-citationTuning electronic correlations in transition metal pnictides: Chemistry beyond the valence count
Razzoli, E., Matt, C. E., Kobayashi, M., Wang, X.-P., Strocov, V. N., van Roekeghem, A., Biermann, S., Plumb, N. C., Radovic, M., Schmitt, T., et al. (2015) · Physical Review B · doi:10.1103/physrevb.91.214502 · Cited by 25
Self-citationConcept of a multichannel spin-resolving electron analyzer based on Mott scattering
Strocov, V. N., Petrov, V. N., & Dil, J. H. (2015) · Journal of Synchrotron Radiation · doi:10.1107/s160057751500363x · Cited by 25
Self-citationMicroscopic effects of Dy doping in the topological insulator Bi2Te3
Duffy, L. B., Steinke, N., Krieger, J. A., Figueroa, A. I., Kummer, K., Lancaster, T., Giblin, S. R., Pratt, F. L., Blundell, S. J., Prokscha, T., et al. (2018) · Physical review. B./Physical review. B · doi:10.1103/physrevb.97.174427 · Cited by 25
Self-citationRösner, B., Dudin, P., Bosgra, J., Hoesch, M., & Dávid, C. (2019) · Journal of Synchrotron Radiation · doi:10.1107/s1600577519000869 · Cited by 25
Strain-Induced Anion-Site Occupancy in Perovskite Oxyfluoride Films
Wang, J., Shin, Y., Paudel, J. R., Grassi, J., Sah, R. K., Yang, W., Karapetrova, E., Zaidan, A., Strocov, V. N., Klewe, C., et al. (2021) · Chemistry of Materials · doi:10.1021/acs.chemmater.0c04793 · Cited by 24
Self-citationSoft X-ray ARPES for three-dimensional crystals in the micrometre region
Muro, T., Senba, Y., Ohashi, H., Ohkochi, T., Matsushita, T., KINOSHITA, T., & Shin, S. (2021) · Journal of Synchrotron Radiation · doi:10.1107/s1600577521007487 · Cited by 24
Tunable spin helical Dirac quasiparticles on the surface of three-dimensional HgTe
Liu, C., Bian, G., Chang, T., Wang, K., Xu, S., Belopolski, I., Miotkowski, I., Cao, H., Miyamoto, K., Xu, C., et al. (2015) · Physical Review B · doi:10.1103/physrevb.92.115436 · Cited by 23
Self-citationHuang, D., Nakamura, H., Küster, K., Yaresko, A., Samal, D., Schröter, N. B. M., Strocov, V. N., Starke, U., & Takagi, H. (2019) · Physical Review Materials · doi:10.1103/physrevmaterials.3.124203 · Cited by 23
Self-citationYáng, X., LaBollita, H., Cheng, Z., Bhandari, H., Cochran, T. A., Yin, J., Hossain, M. S., Belopolski, I., Zhang, Q., Jiang, Y.-X., et al. (2022) · Physical review. B./Physical review. B · doi:10.1103/physrevb.105.l121107 · Cited by 22
Self-citationGiant Room‐Temperature Topological Hall Effect in a Square‐Net Ferromagnet LaMn 2 Ge 2
Roychowdhury, S., Yanda, P., Samanta, K., Yi, C., Yao, M., Orlandi, F., Manuel, P., Khalyavin, D. D., Valle, E. D., Constantinou, P., et al. (2024) · Advanced Materials · doi:10.1002/adma.202305916 · Cited by 22
Self-citationInterplay between disorder and electronic correlations in compositionally complex alloys
Redka, D. S., Khan, S. A., Martino, E., Mettan, X., Ćirić, L., Tolj, D., Ivšić, T., Held, A., Caputo, M., Guedes, E. B., et al. (2024) · Nature Communications · doi:10.1038/s41467-024-52349-8 · Cited by 22
Self-citationProtagonists and spectators during photocatalytic solar water splitting with SrTaO x N y oxynitride
Lawley, C., Tehrani, Z. P., Clark, A. H., Safonova, О. V., Döbeli, M., Strocov, V. N., Schmidt, T. J., Lippert, T. K., Nachtegaal, M., & Pergolesi, D. (2021) · Journal of Materials Chemistry A · doi:10.1039/d1ta05052d · Cited by 21
Self-citationBulk Dirac cone and highly anisotropic electronic structure of Ni Te 2
Nurmamat, M., Eremeev, S. V., Wang, X., Yoshikawa, T., Kono, T., Kakoki, M., Muro, T., Jiang, Q., Sun, Z., Ye, M., et al. (2021) · Physical review. B./Physical review. B · doi:10.1103/physrevb.104.155133 · Cited by 21
Self-citationVisualizing Higher-Fold Topology in Chiral Crystals
Cochran, T. A., Belopolski, I., Manna, K., Yahyavi, M., Liu, Y., Sanchez, D. S., Cheng, Z., Yáng, X., Multer, D., Yin, J., et al. (2023) · Physical Review Letters · doi:10.1103/physrevlett.130.066402 · Cited by 21
Self-citationYu, T., Wright, J. G., Khalsa, G., Pamuk, B., Chang, C. S., Matveyev, Y., Wang, X., Schmitt, T., Feng, D. L., Muller, D. A., et al. (2021) · Science Advances · doi:10.1126/sciadv.abi5833 · Cited by 20
Self-citationDerondeau, G., Bisti, F., Kobayashi, M., Braun, J., Ebert, H., Rogalev, V. A., Shi, M., Schmitt, T., Ma, J., Ding, H., et al. (2017) · Scientific Reports · doi:10.1038/s41598-017-09480-y · Cited by 20
Self-citationTakeda, T., Suzuki, M., Anh, L. Đ., Tu, N. T., Schmitt, T., Yoshida, S., Sakano, M., Ishizaka, K., Takeda, Y., Fijimori, S.-I., et al. (2020) · Physical review. B./Physical review. B · doi:10.1103/physrevb.101.155142 · Cited by 20
Self-citationBerner, G., Sing, M., Pfaff, F., Benckiser, E., Wu, M. Q., Christiani, G., Logvenov, G. Y., Habermeier, H. ‐., Kobayashi, M., Strocov, V. N., et al. (2015) · Physical Review B · doi:10.1103/physrevb.92.125130 · Cited by 19
Self-citationWan, Q., Yang, T., Li, S.-F., Yang, M., Zhu, Z., Wu, C., Peng, C., Mo, S., Wu, W., Chen, Z., et al. (2021) · Physical review. B./Physical review. B · doi:10.1103/physrevb.103.165107 · Cited by 19
Self-citationElectrons and Polarons at Oxide Interfaces Explored by Soft-X-Ray ARPES
Strocov, V. N., Cancellieri, C., & Mishchenko, A. S. (2018) · Springer series in materials science · doi:10.1007/978-3-319-74989-1_6 · Cited by 19
Self-citationDepth-resolved charge reconstruction at the LaNiO3/CaMnO3 interface
Chandrasena, R. U., Flint, C. L., Yang, W.-S., Arab, A., Nemšák, S., Gehlmann, M., Özdöl, V. B., Bisti, F., Wijesekara, K. D., Meyer-Ilse, J., et al. (2018) · Physical review. B./Physical review. B · doi:10.1103/physrevb.98.155103 · Cited by 18
Self-citationExperimental Band Structure of Pb(Zr,Ti)O3: Mechanism of Ferroelectric Stabilization
Popescu, D. G., Huşanu, M. A., Constantinou, P., Filip, L. D., Trupină, L., Bucur, C. I., Pasuk, I., Chirilă, C., Hrib, L., Stancu, V., et al. (2023) · Advanced Science · doi:10.1002/advs.202205476 · Cited by 17
Self-citationProbing the interlayer coupling in 2H−NbS2 via soft x-ray angle-resolved photoemission spectroscopy
Huang, D., Nakamura, H., Küster, K., Wedig, U., Schröter, N. B. M., Strocov, V. N., Starke, U., & Takagi, H. (2022) · Physical review. B./Physical review. B · doi:10.1103/physrevb.105.245145 · Cited by 16
Self-citationTunable topologically driven Fermi arc van Hove singularities
Sanchez, D. S., Cochran, T. A., Belopolski, I., Cheng, Z., Yáng, X., Liu, Y., Hou, T., Xu, X., Manna, K., Shekhar, C., et al. (2023) · Nature Physics · doi:10.1038/s41567-022-01892-6 · Cited by 16
Self-citationThin-film TaAs: Developing a platform for Weyl semimetal devices
Nelson, J. N., Rice, A. D., Kurleto, R., Shackelford, A., Sierzega, Z., Hao, P., Berggren, B. S., Jiang, C., Norman, A. G., Holtz, M. E., et al. (2023) · Matter · doi:10.1016/j.matt.2023.06.018 · Cited by 16
Momentum-resolved electronic structure of LaTiO2N photocatalysts by resonant Soft-X-ray ARPES
Lawley, C., Arab, A., Hartl, A., Staykov, A., Döbeli, M., Schmitt, T., Pergolesi, D., Lippert, T. K., & Strocov, V. N. (2023) · Communications Materials · doi:10.1038/s43246-023-00344-9 · Cited by 15
Self-citationTsai, H.-M., Fu, H., Kuo, C., Huang, L.-J., Lee, C. S., Hua, C.-Y., Kao, K.-Y., Lin, H., Fung, H., Chung, S.-C., et al. (2019) · AIP conference proceedings · doi:10.1063/1.5084678 · Cited by 15
Kobayashi, M., Anh, L. D., Minář, J., Khan, W., Borek, S., Hai, P. N., Harada, Y., Schmitt, T., Oshima, M., Fujimori, A., et al. (2021) · Physical review. B./Physical review. B · doi:10.1103/physrevb.103.115111 · Cited by 15
Self-citationHard X-ray Photoemission: An Overview and Future Perspective
Fadley, C. S. (2015) · Springer series in surface sciences · doi:10.1007/978-3-319-24043-5_1 · Cited by 14
Yu, T., Xu, M., Yang, W., Song, Y., Wen, C., Yao, Q., Lou, X. N., Zhang, T., Li, W., Wei, X., et al. (2022) · Nature Communications · doi:10.1038/s41467-022-34254-0 · Cited by 14
Self-citationVydrovà, Z., Schwier, E. F., Monney, G., Jaouen, T., Razzoli, E., Monney, C., Hildebrand, B., Didiot, C., Berger, H., Schmitt, T., et al. (2015) · Physical Review B · doi:10.1103/physrevb.91.235129 · Cited by 14
Self-citationSchönhense, G., & Elmers, H. J. (2022) · Journal of Vacuum Science & Technology A Vacuum Surfaces and Films · doi:10.1116/6.0001500 · Cited by 13
Kume, T., Hiraguri, K., Imamura, Y., Matsuzawa, Y., Saito, T., Miyashita, H., Takeo, Y., Senba, Y., Kishimoto, H., Ohashi, H., et al. (2022) · Review of Scientific Instruments · doi:10.1063/5.0087171 · Cited by 13
Metadata
- Authors
- Strocov, V. N., Wang, X., Shi, M., Kobayashi, M., Krempasky, J., Hess, C., Schmitt, T., & Patthey, L.
- Affiliations
- Paul Scherrer Institute (CH)
- Venue
- Journal of Synchrotron Radiation
- Published
- 2013-11-07
- Volume
- 21
- Issue
- 1
- Pages
- 32-44
- ISSN
- 0909-0495 (ISSN-L)
- 1600-5775
- OpenAlex
- W2051471521
- Semantic Scholar
- e7cede113a9234604de162a75218b30db0f598a8
- Cited by
- 163
- References
- 35
- Citations by year
- 2026: 4 · 2025: 9 · 2024: 15 · 2023: 15 · 2022: 18 · 2021: 15 · 2020: 13 · 2019: 18 · 2018: 13 · 2017: 16 · 2016: 12 · 2015: 13 · 2014: 2
- FWCI
- 3.56
- Type
- journal article
- Language
- en
- Open access
- bronze
- doi.org
- Licence
- Locations
- Journal of Synchrotron Radiation (publishedVersion)
- PubMed (publishedVersion)
- DORA PSI (Paul Scherrer Institute) (submittedVersion, other-oa)
- Topics
- Physical Sciences › Materials Science › Surfaces, Coatings and Films › Electron and X-Ray Spectroscopy Techniques
- Physical Sciences › Physics and Astronomy › Radiation › X-ray Spectroscopy and Fluorescence Analysis
- Physical Sciences › Physics and Astronomy › Radiation › Advanced X-ray Imaging Techniques
- Keywords
- soft X-ray ARPES, grazing incidence, beam alignment, angular resolution, buried heterostructure, resonant excitation
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