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Oxygen-Mediated Diffusion of Oxygen Vacancies on the TiO 2 (110) Surface
Abstract
Defects such as oxygen vacancies play a crucial role in the surface properties of transition metal oxides. By means of time-resolved, high-resolution scanning tunneling microscopy, we unraveled an adsorbate-mediated diffusion mechanism of oxygen vacancies on rutile TiO 2 (110). Adsorbed oxygen molecules mediate vacancy diffusion through the loss of an oxygen atom to a vacancy and the sequential capture of an oxygen atom from a neighboring bridging oxygen row, leading to an anisotropic oxygen vacancy diffusion pathway perpendicular to the bridging oxygen rows.
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Cites
Photocatalysis on TiO2 Surfaces: Principles, Mechanisms, and Selected Results
Linsebigler, A. L., Lu, G., & Yates, J. T. (1995) · Chemical Reviews · doi:10.1021/cr00035a013 · Cited by 11,575
Cited by
TiO2 photocatalysis and related surface phenomena
FUJISHIMA, A., ZHANG, X., & TRYK, D. (2008) · Surface Science Reports · doi:10.1016/j.surfrep.2008.10.001 · Cited by 6,737
Surface Science Studies of the Photoactivation of TiO 2 New Photochemical Processes
Thompson, T. L., & Yates, J. T. (2006) · Chemical Reviews · doi:10.1021/cr050172k · Cited by 2,064
Defect Chemistry of Nonprecious‐Metal Electrocatalysts for Oxygen Reactions
Yan, D., Li, Y., Huo, J., Chen, R., Dai, L., & Wang, S. (2017) · Advanced Materials · doi:10.1002/adma.201606459 · Cited by 1,600
Ganduglia-Pirovano, M. V., Hofmann, A., & Sauer, J. (2007) · Surface Science Reports · doi:10.1016/j.surfrep.2007.03.002 · Cited by 1,284
The roles of oxygen vacancies in electrocatalytic oxygen evolution reaction
Zhu, K., Shi, F., Zhu, X., & Yang, W. (2020) · Nano Energy · doi:10.1016/j.nanoen.2020.104761 · Cited by 1,018
Metadata
- Authors
- Schaub, R., Wahlström, E., Rønnau, A., Lægsgaard, E., Stensgaard, I., & Besenbacher, F.
- Venue
- Science
- Published
- 2003-01-17
- Volume
- 299
- Issue
- 5605
- Pages
- 377-379
- ISSN
- 0036-8075 (ISSN-L)
- 1095-9203
- OpenAlex
- W1967927080
- Cited by
- 466
- References
- 1
- FWCI
- 27.27
- Type
- journal article
- Language
- en
- Open access
- closed
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- Schaub, R., Wahlström, E., Rønnau, A., Lægsgaard, E., Stensgaard, I., & Besenbacher, F. (2003). Oxygen-Mediated Diffusion of Oxygen Vacancies on the TiO 2 (110) Surface. Science. https://doi.org/10.1126/science.1078962
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
Semantic Scholar’s data is described in: Kinney, R., et al. (2023). The Semantic Scholar Open Data Platform. arXiv:2301.10140.
