The DOI matches its Crossref record; 17 of the 17 references it cites were found in a registry or an index.
Defect Chemistry of Nonprecious‐Metal Electrocatalysts for Oxygen Reactions
Abstract
Oxygen electrocatalysis, including the oxygen‐reduction reaction (ORR) and oxygen‐evolution reaction (OER), is a critical process for metal–air batteries. Therefore, the development of electrocatalysts for the OER and the ORR is of essential importance. Indeed, various advanced electrocatalysts have been designed for the ORR or the OER; however, the origin of the advanced activity of oxygen electrocatalysts is still somewhat controversial. The enhanced activity is usually attributed to the high surface areas, the unique facet structures, the enhanced conductivities, or even to unclear synergistic effects, but the importance of the defects, especially the intrinsic defects, is often neglected. More recently, the important role of defects in oxygen electrocatalysis has been demonstrated by several groups. To make the defect effect clearer, the recent development of this concept is reviewed here and a novel principle for the design of oxygen electrocatalysts is proposed. An overview of the defects in carbon‐based, metal‐free electrocatalysts for ORR and various defects in metal oxides/selenides for OER is also provided. The types of defects and controllable strategies to generate defects in electrocatalysts are presented, along with techniques to identify the defects. The defect–activity relationship is also explored by theoretical methods.
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Cites
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Cited by
Xiao, Z., Huang, Y.-C., Dong, C.-L., Xie, C., Liu, Z., Du, S., Chen, W., Yan, D., Tao, L., Shu, Z., et al. (2020) · Journal of the American Chemical Society · doi:10.1021/jacs.0c00257 · Cited by 1,445
Self-citationHeterostructures for Electrochemical Hydrogen Evolution Reaction: A Review
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Defect Engineering on Electrode Materials for Rechargeable Batteries
Zhang, Y., Tao, L., Xie, C., Wang, D., Zou, Y., Chen, R., Wang, Y., Jia, C., & Wang, S. (2020) · Advanced Materials · doi:10.1002/adma.201905923 · Cited by 1,019
Self-citationHighly selective oxygen reduction to hydrogen peroxide on transition metal single atom coordination
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Defect engineering in earth-abundant electrocatalysts for CO2 and N2 reduction
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Metadata
- Authors
- Yan, D., Li, Y., Huo, J., Chen, R., Dai, L., & Wang, S.
- Venue
- Advanced Materials
- Publisher
- Wiley
- Published
- 2017-05-16
- Volume
- 29
- Issue
- 48
- ISSN
- 0935-9648 (ISSN-L)
- 1521-4095
- OpenAlex
- W2616187014
- Cited by
- 1,600
- References
- 17
- FWCI
- 49.81
- Type
- journal article
- Language
- en
- Open access
- closed
- Funders
- National Natural Science Foundation of China (51402100, 21573066)
- Natural Science Foundation of Hunan Province (2016JJ1006, 2016TP1009)
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