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Electronic Structure Control of Single-Walled Carbon Nanotube Functionalization
Abstract
Diazonium reagents functionalize single-walled carbon nanotubes suspended in aqueous solution with high selectivity and enable manipulation according to electronic structure. For example, metallic species are shown to react to the near exclusion of semiconducting nanotubes under controlled conditions. Selectivity is dictated by the availability of electrons near the Fermi level to stabilize a charge-transfer transition state preceding bond formation. The chemistry can be reversed by using a thermal treatment that restores the pristine electronic structure of the nanotube.
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Citations
Cited by
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McCreery, R. L. (2008) · Chemical Reviews · doi:10.1021/cr068076m · Cited by 2,729
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Eder, D. (2010) · Chemical Reviews · doi:10.1021/cr800433k · Cited by 819
Stepwise Quenching of Exciton Fluorescence in Carbon Nanotubes by Single-Molecule Reactions
Cognet, L., Tsyboulski, D. A., Rocha, J.-D. R., Doyle, C. D., Tour, J. M., & Weisman, R. B. (2007) · Science · doi:10.1126/science.1141316 · Cited by 506
Self-citationControlling the optical properties of carbon nanotubes with organic colour-centre quantum defects
Brozena, A. H., Kim, M., Powell, L. R., & Wang, Y. (2019) · Nature Reviews Chemistry · doi:10.1038/s41570-019-0103-5 · Cited by 207
Remotely actuated shape memory effect of electrospun composite nanofibers
Gong, T., Li, W., Chen, H., Wang, L., Shao, S., & Zhou, S. (2012) · Acta Biomaterialia · doi:10.1016/j.actbio.2011.12.006 · Cited by 147
Metadata
- Authors
- Strano, M. S., Dyke, C. A., Usrey, M. L., Barone, P. W., Allen, M. J., Shan, H., Kittrell, C., Hauge, R. H., Tour, J. M., & Smalley, R. E.
- Venue
- Science
- Published
- 2003-09-12
- Volume
- 301
- Issue
- 5639
- Pages
- 1519-1522
- ISSN
- 0036-8075 (ISSN-L)
- 1095-9203
- OpenAlex
- W2039953952
- Cited by
- 1,357
- References
- 0
- FWCI
- 50.86
- Type
- journal article
- Language
- en
- Open access
- closed
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- Strano, M. S., Dyke, C. A., Usrey, M. L., Barone, P. W., Allen, M. J., Shan, H., Kittrell, C., Hauge, R. H., Tour, J. M., & Smalley, R. E. (2003). Electronic Structure Control of Single-Walled Carbon Nanotube Functionalization. Science. https://doi.org/10.1126/science.1087691
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
Semantic Scholar’s data is described in: Kinney, R., et al. (2023). The Semantic Scholar Open Data Platform. arXiv:2301.10140.
