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Wet Electrons at the H 2 O/TiO 2 (110) Surface
Abstract
At interfaces of metal oxide and water, partially hydrated or “wet-electron” states represent the lowest energy pathway for electron transfer. We studied the photoinduced electron transfer at the H 2 O/TiO 2 (110) interface by means of time-resolved two-photon photoemission spectroscopy and electronic structure theory. At ∼1-monolayer coverage of water on partially hydroxylated TiO 2 surfaces, we found an unoccupied electronic state 2.4 electron volts above the Fermi level. Density functional theory shows this to be a wet-electron state analogous to that reported in water clusters and which is distinct from hydrated electrons observed on water-covered metal surfaces. The decay of electrons from the wet-electron state to the conduction band of TiO 2 occurs in ≤15 femtoseconds.
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Citations
Cites
Photocatalysis on TiO2 Surfaces: Principles, Mechanisms, and Selected Results
Linsebigler, A. L., Lu, G., & Yates, J. T. (1995) · Chemical Reviews · doi:10.1021/cr00035a013 · Cited by 11,575
The surface science of titanium dioxide
Diebold, U. (2003) · Surface Science Reports · doi:10.1016/s0167-5729(02)00100-0 · Cited by 7,944
Cited by
Fundamentals of TiO2 Photocatalysis: Concepts, Mechanisms, and Challenges
Guo, Q., Zhou, C., Ma, Z., & Yang, X. (2019) · Advanced Materials · doi:10.1002/adma.201901997 · Cited by 1,909
Titanium Dioxide Crystals with Tailored Facets
Liu, G., Yang, H. G., Pan, J., Yang, Y. Q., Lu, G. Q. (., & Cheng, H.-M. (2014) · Chemical Reviews · doi:10.1021/cr400621z · Cited by 1,084
Zheng, Q., Chu, W., Zhao, C., Zhang, L., Guo, H., Wang, Y., Jiang, X., & Zhao, J. (2019) · WIREs Computational Molecular Science · doi:10.1002/wcms.1411 · Cited by 452
Self-citationKetteler, G., Yamamoto, S., Bluhm, H., Andersson, K., Starr, D. E., Ogletree, D. F., Ogasawara, H., Nilsson, A., & Salmeron, M. (2007) · The Journal of Physical Chemistry C · doi:10.1021/jp068606i · Cited by 419
Thermally-driven processes on rutile TiO2(110)-(1×1): A direct view at the atomic scale
Dohnálek, Z., Lyubinetsky, I., & Rousseau, R. (2010) · Progress in Surface Science · doi:10.1016/j.progsurf.2010.03.001 · Cited by 310
Metadata
- Authors
- Onda, K., Li, B., Zhao, J., Jordan, K. D., Yang, J., & Petek, H.
- Venue
- Science
- Published
- 2005-05-20
- Volume
- 308
- Issue
- 5725
- Pages
- 1154-1158
- ISSN
- 0036-8075 (ISSN-L)
- 1095-9203
- OpenAlex
- W1973629646
- Cited by
- 257
- References
- 2
- FWCI
- 12.77
- Type
- journal article
- Language
- en
- Open access
- closed
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- Onda, K., Li, B., Zhao, J., Jordan, K. D., Yang, J., & Petek, H. (2005). Wet Electrons at the H 2 O/TiO 2 (110) Surface. Science. https://doi.org/10.1126/science.1109366
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